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DOI10.1021/acs.est.8b06575
Accumulation of Atmospheric Mercury in Glacier Cryoconite over Western China
Huang, Jie1,2; Kang, Shichang3,9; Ma, Ming4; Guo, Junming3; Cong, Zhiyuan1,2; Dong, Zhiwen3; Yin, Runsheng5; Xu, Jianzhong3; Tripathee, Lekhendra3; Ram, Kirpa1,2,6; Wang, Feiyue7,8
发表日期2019
ISSN0013-936X
EISSN1520-5851
卷号53期号:12页码:6632-6639
英文摘要

Cryoconite is a granular aggregate, comprised of both mineral and biological material, and known to accumulate atmospheric contaminants. In this study, cryoconite was sampled from seven high-elevation glaciers in Western China to investigate the spatial and altitudinal patterns of atmospheric mercury (Hg) accumulation in the cryoconite. The results show that total Hg (Hg-T) concentrations in cryoconite were significant with relatively higher Hg accumulation in the southern glaciers (66.0 +/- 29.3 ng g(-1)), monsoon-influenced regions, than those in the northern glaciers (42.5 +/- 20.7 ng g(-1)), westerlies-influenced regions. The altitudinal profile indicates that Hg-T concentrations in the northern glaciers decrease significantly with altitude, while those in the southern glaciers generally increase toward higher elevations. Unexpectedly high accumulation of methyl-Hg (MeHg) with an average of 1.0 +/- 0.4 ng g(-1) was also detected in the cryoconite samples, revealing the surface of cryoconite could act as a potential site for Hg methylation in alpine environments. Our preliminary estimate suggests a storage of similar to 34.3 +/- 17.4 and 0.65 +/- 0.28 kg of Hg-T and MeHg from a single year of formation process in the glacier cryoconite. Therefore, glacier cryoconite could play an important role in Hg storage and transformation, which may result in downstream effects on glacier-fed ecosystems under climate warming scenario.


WOS研究方向Engineering ; Environmental Sciences & Ecology
来源期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/99207
作者单位1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China;
2.Chinese Acad Sci, CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China;
3.Chinese Acad Sci, Northeast Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China;
4.Southwest Univ, Coll Resources & Environm, Chongqing 400715, Peoples R China;
5.Chinese Acad Sci, Inst Geochem, State Key Lab Ore Deposit Geochem, Guiyang 550002, Guizhou, Peoples R China;
6.Banaras Hindu Univ, Inst Environm & Sustainable Dev, Varanasi 221005, Uttar Pradesh, India;
7.Univ Manitoba, Ctr Earth Observat Sci, Winnipeg, MB R3T 2N2, Canada;
8.Univ Manitoba, Dept Environm & Geog, Winnipeg, MB R3T 2N2, Canada;
9.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Huang, Jie,Kang, Shichang,Ma, Ming,et al. Accumulation of Atmospheric Mercury in Glacier Cryoconite over Western China[J],2019,53(12):6632-6639.
APA Huang, Jie.,Kang, Shichang.,Ma, Ming.,Guo, Junming.,Cong, Zhiyuan.,...&Wang, Feiyue.(2019).Accumulation of Atmospheric Mercury in Glacier Cryoconite over Western China.ENVIRONMENTAL SCIENCE & TECHNOLOGY,53(12),6632-6639.
MLA Huang, Jie,et al."Accumulation of Atmospheric Mercury in Glacier Cryoconite over Western China".ENVIRONMENTAL SCIENCE & TECHNOLOGY 53.12(2019):6632-6639.
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