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DOI10.1002/slct.201900253
Oxygen-Doped Porous Carbon Nanosheet for Efficient N-2 Fixation to NH3 at Ambient Conditions
Chen, Jiayin1; Huang, Hong1; Xia, Li1; Xie, Hongtao1; Ji, Lei1; Wei, Peipei1; Zhao, Runbo1; Chen, Hongyu1; Asiri, Abdullah M.2,3; Sun, Xuping1
发表日期2019
ISSN2365-6549
卷号4期号:12页码:3547-3550
英文摘要

NH3 is one of the largest-volume industrial chemicals synthesized in the world. It not only is a kind of important chemical base materials to produce fertilizers, plastics and explosives, but also can serve as a clean energy carrier with high hydrogen content for a sustainable energy supply. N-2 is the most abundant gas in atmosphere, but its inert character caused by the strong triple bond, impedes itself from being converted to NH3. In nature, this shortcoming is overcome by biological N-2 fixation utilizing nitrogenase enzymes. Industrially, fixation of N-2-to-NH3 prevailingly depends on Haber-Bosch process using Ru- or Fe-based catalysts, but this process consumes large energy and emits heavy carbon which increases crisis of global warming.


WOS研究方向Chemistry
来源期刊CHEMISTRYSELECT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/95222
作者单位1.Univ Elect Sci & Technol China, Inst Fundamental & Frontier Sci, Chengdu 610054, Sichuan, Peoples R China;
2.King Abdulaziz Univ, Fac Sci, Chem Dept, POB 80203, Jeddah 21589, Saudi Arabia;
3.King Abdulaziz Univ, Ctr Excellence Adv Mat Res, POB 80203, Jeddah 21589, Saudi Arabia
推荐引用方式
GB/T 7714
Chen, Jiayin,Huang, Hong,Xia, Li,et al. Oxygen-Doped Porous Carbon Nanosheet for Efficient N-2 Fixation to NH3 at Ambient Conditions[J],2019,4(12):3547-3550.
APA Chen, Jiayin.,Huang, Hong.,Xia, Li.,Xie, Hongtao.,Ji, Lei.,...&Sun, Xuping.(2019).Oxygen-Doped Porous Carbon Nanosheet for Efficient N-2 Fixation to NH3 at Ambient Conditions.CHEMISTRYSELECT,4(12),3547-3550.
MLA Chen, Jiayin,et al."Oxygen-Doped Porous Carbon Nanosheet for Efficient N-2 Fixation to NH3 at Ambient Conditions".CHEMISTRYSELECT 4.12(2019):3547-3550.
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