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DOI10.1029/2017JD028181
Fossil Fuel Combustion Emission From South Asia Influences Precipitation Dissolved Organic Carbon Reaching the Remote Tibetan Plateau: Isotopic and Molecular Evidence
Li, Chaoliu1,2,3; Chen, Pengfei4; Kang, Shichang2,4,5; Yan, Fangping3; Tripathee, Lekhendra4; Wu, Guangjian1,2; Qu, Bin6; Sillanpaa, Mika3; Yang, Di7; Dittmar, Thorsten8; Stubbins, Aron9,10,11,12; Raymond, Peter A.13
发表日期2018
ISSN2169-897X
EISSN2169-8996
卷号123期号:11页码:6248-6258
英文摘要

The dissolved organic carbon in precipitation (water-soluble organic carbon, WSOC) can provide a carbon subsidy to receiving ecosystems. The concentrations, isotopic signatures (C-13/Delta C-14), and molecular signatures (transform ion cyclotron mass spectrometry) of WSOC being delivered to Nam Co-a remote site on the inland Tibetan Plateau (TP)were compared to those of WSOC in the snowpack, and in wet deposition from urban cities fringing the TP. The average WSOC concentration at Nam Co (1.0 +/- 0.9mg C L-1) was lower than for the large cities (1.6 to 2.3mgCL(-1)) but higher than in the snowpack samples (0.26 +/- 0.09mgCL(-1)). Based upon radiocarbon data, it is estimated that 156% of Nam Co WSOC was fossil derived, increasing to 208% for snowpack WSOC, 29 +/- 4% for Lhasa WSOC, and 34 +/- 8% for the three cities. Transform ion cyclotron mass spectrometry results revealed that the abundance of dissolved black carbon and sulfur-containing molecules of WSOC increased in the order Nam Co

语种英语
WOS研究方向Meteorology & Atmospheric Sciences
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
来源机构中国科学院西北资源环境生态研究院
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/89589
作者单位1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing, Peoples R China;;
2.CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing, Peoples R China;;
3.Lappeenranta Univ Technol, Lab Green Chem, Mikkeli, Finland;;
4.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou, Gansu, Peoples R China;;
5.Univ CAS, Beijing, Peoples R China;;
6.Nanjing Univ Informat Sci & Technol, Int Joint Lab Climate & Environm Change, Yale NUIST Ctr Atmospher Environm, Nanjing, Jiangsu, Peoples R China;;
7.Chengdu Univ Technol, State Key Lab Oil & Gas Reservoir Geol & Exploita, Chengdu, Sichuan, Peoples R China;;
8.Carl Von Ossietzky Univ Oldenburg, Inst Chem & Biol Marine Environm, ICBM MPI Bridging Grp, Res Grp Marine Geochem, Oldenburg, Germany;;
9.Northeastern Univ, Dept Marine Sci, Boston, MA 02115 USA;;
10.Northeastern Univ, Dept Environm Sci, Boston, MA 02115 USA;;
11.Northeastern Univ, Dept Civil & Environm Engn, Boston, MA 02115 USA;;
12.Northeastern Univ, Dept Chem & Chem Biol, Boston, MA 02115 USA;;
13.Yale Univ, Sch Forestry & Environm Studies, New Haven, CT 06511 USA
推荐引用方式
GB/T 7714
Li, Chaoliu,Chen, Pengfei,Kang, Shichang,et al. Fossil Fuel Combustion Emission From South Asia Influences Precipitation Dissolved Organic Carbon Reaching the Remote Tibetan Plateau: Isotopic and Molecular Evidence[J]. 中国科学院西北资源环境生态研究院,2018,123(11):6248-6258.
APA Li, Chaoliu.,Chen, Pengfei.,Kang, Shichang.,Yan, Fangping.,Tripathee, Lekhendra.,...&Raymond, Peter A..(2018).Fossil Fuel Combustion Emission From South Asia Influences Precipitation Dissolved Organic Carbon Reaching the Remote Tibetan Plateau: Isotopic and Molecular Evidence.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,123(11),6248-6258.
MLA Li, Chaoliu,et al."Fossil Fuel Combustion Emission From South Asia Influences Precipitation Dissolved Organic Carbon Reaching the Remote Tibetan Plateau: Isotopic and Molecular Evidence".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 123.11(2018):6248-6258.
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