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DOI10.1021/es505968b
Differences Between Magnitudes and Health Impacts of BC Emissions Across the United States Using 12 km Scale Seasonal Source Apportionment
Turner, Matthew D.1; Henze, Daven K.1; Hakami, Amir2; Zhao, Shunliu2; Resler, Jaroslav3; Carmichael, Gregory R.4; Stanier, Charles O.4; Baek, Jaemeen4; Sandu, Adrian5; Russell, Armistead G.6; Nenes, Athanasios7,8; Jeong, Gill-Ran7,13; Capps, Shannon L.8,10; Percell, Peter B.9; Pinder, Rob W.10; Napelenok, Sergey L.10; Bash, Jesse O.10; Chai, Tianfeng11,12
发表日期2015-04-07
ISSN0013-936X
卷号49期号:7页码:4362-4371
英文摘要

Recent assessments have analyzed the health impacts of PM2.5 from emissions from different locations and sectors using simplified or reduced-form air quality models. Here we present an alternative approach using the adjoint of the Community Multiscale Air Quality (CMAQ) model, which provides sourcereceptor relationships at highly resolved sectoral, spatial, and temporal scales. While damage resulting from anthropogenic emissions of BC is strongly correlated with population and premature death, we found little correlation between damage and emission magnitude, suggesting that controls on the largest emissions may not be the most efficient means of reducing damage resulting from anthropogenic BC emissions. Rather, the best proxy for locations with damaging BC emissions is locations where premature deaths occur. Onroad diesel and nonroad vehicle emissions are the largest contributors to premature deaths attributed to exposure to BC, while onroad gasoline emissions cause the highest deaths per amount emitted. Emissions in fall and winter contribute to more premature deaths (and more per amount emitted) than emissions in spring and summer. Overall, these results show the value of the high-resolution source attribution for determining the locations, seasons, and sectors for which BC emission controls have the most effective health benefits.


语种英语
WOS记录号WOS:000352659000043
来源期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/61895
作者单位1.Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA;
2.Carleton Univ, Dept Civil & Environm Engn, Ottawa, ON K1S 5B6, Canada;
3.Inst Comp Sci, Nonlinear Modeling, Prague 18207, Czech Republic;
4.Univ Iowa, Dept Chem & Biochem Engn, Iowa City, IA 52242 USA;
5.Virginia Tech, Comp Sci, Blacksburg, VA 24061 USA;
6.Georgia Tech, Sch Civil & Environm Engn, Atlanta, GA 30332 USA;
7.Georgia Tech, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA;
8.Georgia Tech, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA;
9.Univ Houston, Dept Geosci, Houston, TX 77004 USA;
10.US EPA, Atmospher Modeling & Anal Div, Res Triangle Pk, NC 27711 USA;
11.Univ Maryland, Coll Comp Math & Nat Sci, College Pk, MD 20742 USA;
12.NOAA, Air Resources Lab, College Pk, MD 20740 USA;
13.Korea Inst Atmospher Predict Syst, Seoul 156849, South Korea
推荐引用方式
GB/T 7714
Turner, Matthew D.,Henze, Daven K.,Hakami, Amir,et al. Differences Between Magnitudes and Health Impacts of BC Emissions Across the United States Using 12 km Scale Seasonal Source Apportionment[J]. 美国环保署,2015,49(7):4362-4371.
APA Turner, Matthew D..,Henze, Daven K..,Hakami, Amir.,Zhao, Shunliu.,Resler, Jaroslav.,...&Chai, Tianfeng.(2015).Differences Between Magnitudes and Health Impacts of BC Emissions Across the United States Using 12 km Scale Seasonal Source Apportionment.ENVIRONMENTAL SCIENCE & TECHNOLOGY,49(7),4362-4371.
MLA Turner, Matthew D.,et al."Differences Between Magnitudes and Health Impacts of BC Emissions Across the United States Using 12 km Scale Seasonal Source Apportionment".ENVIRONMENTAL SCIENCE & TECHNOLOGY 49.7(2015):4362-4371.
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