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DOI10.1016/j.atmosenv.2015.09.017
Stable isotopes of lead and strontium as tracers of sources of airborne particulate matter in Kyrgyzstan
Dewan, Nitika1; Majestic, Brian J.1; Ketterer, Michael E.2; Miller-Schulze, Justin P.3; Shafer, Martin M.4,5; Schauer, James J.4,5; Solomon, Paul A.6; Artamonova, Maria7; Chen, Boris B.8; Imashev, Sanjar A.8; Carmichael, Greg R.9
发表日期2015-11-01
ISSN1352-2310
卷号120页码:438-446
英文摘要

Central Asia is dominated by an arid climate and desert-like conditions, leading to the potential for long-range transport of desert dust within and out of the region. Of particular interest is the Aral Sea, which has receded in size largely due to water diversion. As a result, newly exposed sediments are resuspended by wind and thus, may be a potential new source of particulate matter within the region. Here, strontium and lead stable isotope ratios are employed along with detailed elemental composition, to explore the contribution of long-range transport of Aral Sea sediments, as well as other potential sources of dust, within Central Asia. Ambient Mho samples were collected during dust and non-dust events from mid-2008 to mid-2009 at two sites in Kyrgyzstan located 1200 and 1500 km ESE of the Aral Sea. Aral Sea sediments and local Kyrgyzstan soils were resuspended and sized to PM10. The Aral Sea sediments have an average Sr-87/Sr-86 ratio of 0.70992. In contrast, the Sr isotope ratio in local soils exhibits an average ratio of 0.71579. Ambient PMio collected in Kyrgyzstan has an average Sr-87/Sr-86 ratio of 0.71177, falling between the values of these two potential sources and indicating a complex mixture of contributing sources. At both sites, airborne Sr isotope ratios measured during dust events were similar, suggesting that Aral Sea sediments only minimally affect air quality in Kyrgyzstan. Elemental analysis and Pb isotope ratios supported this finding. While the Pb isotopes and elemental data both indicate an anthropogenic source, long-range dust transport from other deserts inside and outside the region cannot be ruled out as sources of PM10 in Central Asia. (C) 2015 Elsevier Ltd. All rights reserved.


英文关键词Air pollution;Soils;PM10;Sediments;Dust Long-range transport;Strontium (Sr) isotopes;Lead (Pb) isotopes;Aral Sea;Central Asia
语种英语
WOS记录号WOS:000364255700045
来源期刊ATMOSPHERIC ENVIRONMENT
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/61689
作者单位1.Univ Denver, Dept Chem & Biochem, Denver, CO 80208 USA;
2.Metropolitan State Univ Denver, Dept Chem, Denver, CO 80204 USA;
3.Calif State Univ Sacramento, Dept Chem, Sacramento, CA 95819 USA;
4.Univ Wisconsin, Wisconsin State Lab Hyg, Madison, WI 53718 USA;
5.Univ Wisconsin, Environm Chem & Technol Program, Madison, WI 53706 USA;
6.US EPA, Off Res & Dev, Las Vegas, NV 89193 USA;
7.Inst Atmospher Phys, Moscow 109017, Russia;
8.Kyrgyz Russian Slav Univ, Bishkek 720000, Kyrgyzstan;
9.Univ Iowa, Dept Chem & Biochem Engn, Iowa City, IA 52242 USA
推荐引用方式
GB/T 7714
Dewan, Nitika,Majestic, Brian J.,Ketterer, Michael E.,et al. Stable isotopes of lead and strontium as tracers of sources of airborne particulate matter in Kyrgyzstan[J]. 美国环保署,2015,120:438-446.
APA Dewan, Nitika.,Majestic, Brian J..,Ketterer, Michael E..,Miller-Schulze, Justin P..,Shafer, Martin M..,...&Carmichael, Greg R..(2015).Stable isotopes of lead and strontium as tracers of sources of airborne particulate matter in Kyrgyzstan.ATMOSPHERIC ENVIRONMENT,120,438-446.
MLA Dewan, Nitika,et al."Stable isotopes of lead and strontium as tracers of sources of airborne particulate matter in Kyrgyzstan".ATMOSPHERIC ENVIRONMENT 120(2015):438-446.
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