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DOI10.1038/ncomms13444
Contribution of Arctic seabird-colony ammonia to atmospheric particles and cloud-albedo radiative effect
Croft, B.1; Wentworth, G. R.2,9; Martin, R. V.1,3; Leaitch, W. R.4; Murphy, J. G.2; Murphy, B. N.5,6,8; Kodros, J. K.7; Abbatt, J. P. D.2; Pierce, J. R.1,7
发表日期2016-11-15
ISSN2041-1723
卷号7
英文摘要

The Arctic region is vulnerable to climate change and able to affect global climate. The summertime Arctic atmosphere is pristine and strongly influenced by natural regional emissions, which have poorly understood climate impacts related to atmospheric particles and clouds. Here we show that ammonia from seabird-colony guano is a key factor contributing to bursts of newly formed particles, which are observed every summer in the near-surface atmosphere at Alert, Nunavut, Canada. Our chemical-transport model simulations indicate that the pan-Arctic seabird-influenced particles can grow by sulfuric acid and organic vapour condensation to diameters sufficiently large to promote pan-Arctic cloud-droplet formation in the clean Arctic summertime. We calculate that the resultant cooling tendencies could be large (about -0.5Wm(-2) pan-Arctic-mean cooling), exceeding -1Wm(-2) near the largest seabird colonies due to the effects of seabird-influenced particles on cloud albedo. These coupled ecological-chemical processes may be susceptible to Arctic warming and industrialization.


语种英语
WOS记录号WOS:000387972500001
来源期刊NATURE COMMUNICATIONS
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/61655
作者单位1.Dalhousie Univ, Dept Phys & Atmospher Sci, 6310 Coburg Rd, Halifax, NS B3H 4R2, Canada;
2.Univ Toronto, Dept Chem, 80 St George St, Toronto, ON M5S 3H6, Canada;
3.Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA;
4.Environm & Climate Change Canada, Div Climate Res, 4905 Dufferin St, Toronto, ON M3H 5T4, Canada;
5.Stockholm Univ, Dept Environm Sci & Analyt Chem ACES, Svante Arrhenius Vag 8, SE-11418 Stockholm, Sweden;
6.Stockholm Univ, Bolin Ctr Climate Res, Svante Arrhenius Vag 8, SE-11418 Stockholm, Sweden;
7.Colorado State Univ, Dept Atmospher Sci, 3915W Laporte, Ft Collins, CO 80523 USA;
8.US EPA, Computat Exposure Div, 200 Pk Dr, Res Triangle Pk, NC 27709 USA;
9.Alberta Environm & Pk, Environm Monitoring & Sci Div, 9888 Jasper Ave NW, Edmonton, AB T5J 5C6, Canada
推荐引用方式
GB/T 7714
Croft, B.,Wentworth, G. R.,Martin, R. V.,et al. Contribution of Arctic seabird-colony ammonia to atmospheric particles and cloud-albedo radiative effect[J]. 美国环保署,2016,7.
APA Croft, B..,Wentworth, G. R..,Martin, R. V..,Leaitch, W. R..,Murphy, J. G..,...&Pierce, J. R..(2016).Contribution of Arctic seabird-colony ammonia to atmospheric particles and cloud-albedo radiative effect.NATURE COMMUNICATIONS,7.
MLA Croft, B.,et al."Contribution of Arctic seabird-colony ammonia to atmospheric particles and cloud-albedo radiative effect".NATURE COMMUNICATIONS 7(2016).
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