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DOI10.1016/j.envpol.2018.04.085
Light absorption of organic carbon emitted from burning wood, charcoal, and kerosene in household cookstoves
Xie, Mingjie1,2,3,4; Shen, Guofeng3,4; Holder, Amara L.4; Hays, Michael D.4; Jetter, James J.4
发表日期2018-09-01
ISSN0269-7491
卷号240页码:60-67
英文摘要

Household cookstove emissions are an important source of carbonaceous aerosols globally. The light-absorbing organic carbon (OC), also termed brown carbon (BrC), from cookstove emissions can impact the Earth's radiative balance, but is rarely investigated. In this work, PM2.5 filter samples were collected during combustion experiments with red oak wood, charcoal, and kerosene in a variety of cookstoves mainly at two water boiling test phases (cold start CS, hot start HS). Samples were extracted in methanol and extracts were examined using spectrophotometry. The mass absorption coefficients (MAC(lambda), m(2) g(-1)) at five wavelengths (365, 400, 450, 500, and 550 nm) were mostly inter-correlated and were used as a measurement proxy for BrC. The MAC(365) for red oak combustion during the CS phase correlated strongly to the elemental carbon (EC)/OC mass ratio, indicating a dependency of BrC absorption on burn conditions. The emissions from cookstoves burning red oak have an average MAC(lambda) 2-6 times greater than those burning charcoal and kerosene, and around 3-4 times greater than that from biomass burning measured in previous studies. These results suggest that residential cookstove emissions could contribute largely to ambient BrC, and the simulation of BrC radiative forcing in climate models for biofuel combustion in cookstoves should be treated specifically and separated from open biomass burning. (C) 2018 Elsevier Ltd. All rights reserved.


英文关键词Brown carbon;Cookstove combustion;Mass absorption coefficient;Burn condition
语种英语
WOS记录号WOS:000438322100008
来源期刊ENVIRONMENTAL POLLUTION
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/59980
作者单位1.Nanjing Univ Informat Sci & Technol, Sch Environm Sci & Engn, Jiangsu Key Lab Atmospher Environm Monitoring & P, Collaborat Innovat Ctr Atmospher Environm & Equip, 219 Ningliu Rd, Nanjing 210044, Jiangsu, Peoples R China;
2.Nanjing Univ, State Key Lab Pollut Control & Resource Reuse, Nanjing 210023, Jiangsu, Peoples R China;
3.US EPA, Off Res & Dev, ORISE, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA;
4.US EPA, Off Res & Dev, Natl Risk Management Res Lab, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA
推荐引用方式
GB/T 7714
Xie, Mingjie,Shen, Guofeng,Holder, Amara L.,et al. Light absorption of organic carbon emitted from burning wood, charcoal, and kerosene in household cookstoves[J]. 美国环保署,2018,240:60-67.
APA Xie, Mingjie,Shen, Guofeng,Holder, Amara L.,Hays, Michael D.,&Jetter, James J..(2018).Light absorption of organic carbon emitted from burning wood, charcoal, and kerosene in household cookstoves.ENVIRONMENTAL POLLUTION,240,60-67.
MLA Xie, Mingjie,et al."Light absorption of organic carbon emitted from burning wood, charcoal, and kerosene in household cookstoves".ENVIRONMENTAL POLLUTION 240(2018):60-67.
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