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DOI10.5094/APR.2013.017
Gaseous oxidized mercury dry deposition measurements in the Four Corners area and Eastern Oklahoma, U.S.A.
Sather, Mark E.1; Mukerjee, Shaibal2; Smith, Luther3; Mathew, Johnson4; Jackson, Clarence4; Callison, Ryan5; Scrapper, Larry5; Hathcoat, April5; Adam, Jacque5; Keese, Danielle5; Ketcher, Philip5; Brunette, Robert6; Karlstrom, Jason6; Van der Jagt, Gerard6
发表日期2013-04-01
ISSN1309-1042
卷号4期号:2页码:168-180
英文摘要

Gaseous oxidized mercury (GOM) dry deposition measurements using surrogate surface passive samplers were collected in the Four Corners area and eastern Oklahoma from August, 2009-August, 2011. Using data from a six site area network, a characterization of the magnitude and spatial extent of ambient mercury pollution in the arid Four Corners area was accomplished, which included the observation of a strong regional signature in the GOM dry deposition data set. GOM dry deposition rate estimates ranged from 0.4-1.0 ng/m(2) h at the six Four Corners area monitoring sites, while the GOM dry deposition rate estimate at the eastern Oklahoma monitoring site was lower at 0.2 ng/m(2) h. The highest GOM dry deposition estimates were recorded during the spring and summer while the lowest GOM dry deposition estimates were recorded during the fall and winter. During the second year of this study the highest annual GOM dry deposition estimate so far measured in the United States (U.S.) with smooth-edge surrogate surface passive samplers, 10 889 ng/m(2), was recorded at the Mesa Verde National Park site, a site at which the two-year cumulative GOM dry deposition estimate exceeded the mercury wet deposition estimate. GOM dry deposition estimates during the second year of the study were statistically significantly higher than the first year of the study at six of the seven sites. The data from this study provide a two-year baseline of GOM dry deposition data in the Four Corners area and eastern Oklahoma immediately before the current implementation of new U.S. power plant and boiler mercury control regulations which will significantly reduce mercury emissions from those two sectors of local and regional anthropogenic mercury emission sources.


英文关键词Air pollution;arid area;surrogate surface passive sampling
语种英语
WOS记录号WOS:000318686600005
来源期刊ATMOSPHERIC POLLUTION RESEARCH
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/59848
作者单位1.US Environm Protect Agcy EPA Reg 6, Air Qual Anal Sect, Dallas, TX 75202 USA;
2.US EPA E205 03, Natl Exposure Res Lab, Res Triangle Pk, NC 27711 USA;
3.Alion Sci & Technol Inc, Res Triangle Pk, NC 27709 USA;
4.US EPA Reg 6, Houston Lab, Houston, TX 77099 USA;
5.Cherokee Nation Environm Programs, Tahlequah, OK 74464 USA;
6.Frontier Global Sci, Bothell, WA 98011 USA
推荐引用方式
GB/T 7714
Sather, Mark E.,Mukerjee, Shaibal,Smith, Luther,et al. Gaseous oxidized mercury dry deposition measurements in the Four Corners area and Eastern Oklahoma, U.S.A.[J]. 美国环保署,2013,4(2):168-180.
APA Sather, Mark E..,Mukerjee, Shaibal.,Smith, Luther.,Mathew, Johnson.,Jackson, Clarence.,...&Van der Jagt, Gerard.(2013).Gaseous oxidized mercury dry deposition measurements in the Four Corners area and Eastern Oklahoma, U.S.A..ATMOSPHERIC POLLUTION RESEARCH,4(2),168-180.
MLA Sather, Mark E.,et al."Gaseous oxidized mercury dry deposition measurements in the Four Corners area and Eastern Oklahoma, U.S.A.".ATMOSPHERIC POLLUTION RESEARCH 4.2(2013):168-180.
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