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DOI10.1016/j.jes.2015.05.010
Deposition behavior of residual aluminum in drinking water distribution system: Effect of aluminum speciation
Zhang, Yue1; Shi, Baoyou1; Zhao, Yuanyuan1; Yan, Mingquan2; Lytle, Darren A.3; Wang, Dongsheng1
发表日期2016-04-01
ISSN1001-0742
卷号42页码:142-151
英文摘要

Finished drinking water usually contains some residual aluminum. The deposition of residual aluminum in distribution systems and potential release back to the drinking water could significantly influence the water quality at consumer taps. A preliminary analysis of aluminum content in cast iron pipe corrosion scales and loose deposits demonstrated that aluminum deposition on distribution pipe surfaces could be excessive for water treated by aluminum coagulants including polyaluminum chloride (PACl). In this work, the deposition features of different aluminum species in PACl were investigated by simulated coil-pipe test, batch reactor test and quartz crystal microbalance with dissipation monitoring. The deposition amount of non-polymeric aluminum species was the least, and its deposition layer was soft and hydrated, which indicated the possible formation of amorphous Al(OH)(3). Al-13 had the highest deposition tendency, and the deposition layer was rigid and much less hydrated, which indicated that the deposited aluminum might possess regular structure and self-aggregation of Al-13 could be the main deposition mechanism. While for Al-30, its deposition was relatively slower and deposited aluminum amount was relatively less compared with Al-13. However, the total deposited mass of Al-30 was much higher than that of Al-13, which was attributed to the deposition of particulate aluminum matters with much higher hydration state. Compared with stationary condition, stirring could significantly enhance the deposition process, while the effect of pH on deposition was relatively weak in the near neutral range of 6.7 to 8.7. (C) 2015 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.


英文关键词Aluminum deposition;Drinking water distribution system;Polyaluminum chloride (PACl);Quartz crystal microbalance
语种英语
WOS记录号WOS:000374976500017
来源期刊JOURNAL OF ENVIRONMENTAL SCIENCES
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/59647
作者单位1.Chinese Acad Sci, Key Lab Drinking Water Sci & Technol, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China;
2.Peking Univ, Coll Environm Sci & Engn, Beijing 100871, Peoples R China;
3.US EPA, Cincinnati, OH 45268 USA
推荐引用方式
GB/T 7714
Zhang, Yue,Shi, Baoyou,Zhao, Yuanyuan,et al. Deposition behavior of residual aluminum in drinking water distribution system: Effect of aluminum speciation[J]. 美国环保署,2016,42:142-151.
APA Zhang, Yue,Shi, Baoyou,Zhao, Yuanyuan,Yan, Mingquan,Lytle, Darren A.,&Wang, Dongsheng.(2016).Deposition behavior of residual aluminum in drinking water distribution system: Effect of aluminum speciation.JOURNAL OF ENVIRONMENTAL SCIENCES,42,142-151.
MLA Zhang, Yue,et al."Deposition behavior of residual aluminum in drinking water distribution system: Effect of aluminum speciation".JOURNAL OF ENVIRONMENTAL SCIENCES 42(2016):142-151.
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