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DOI | 10.1016/j.atmosenv.2014.05.041 |
Characterizing reduced sulfur compounds emissions from a swine concentrated animal feeding operation | |
Rumsey, Ian C.1; Aneja, Viney P.1; Lonneman, William A.2 | |
发表日期 | 2014-09-01 |
ISSN | 1352-2310 |
卷号 | 94页码:458-466 |
英文摘要 | Reduced sulfur compounds (RSCs) emissions from concentrated animal feeding operations (CAFOs) have become a potential environmental and human health concern, as a result of changes in livestock production methods. RSC emissions were determined from a swine CAFO in North Carolina. RSC measurements were made over a period of approximate to 1 week from both the barn and lagoon during each of the four seasonal periods from June 2007 to April 2008. During sampling, meteorological and other environmental parameters were measured continuously. Seasonal hydrogen sulfide (H2S) barn concentrations ranged from 72 to 631 ppb. Seasonal dimethyl sulfide (DMS; CH3SCH3) and dimethyl disulfide (DMDS; CH3S2CH3) concentrations were 2-3 orders of magnitude lower, ranging from 0.18 to 0.89 ppb and 0.47 to 1.02 ppb, respectively. The overall average barn emission rate was 3.3 g day(-1) AU(-1) (AU (animal unit) = 500 kg of live animal weight) for H2S, which was approximately two orders of magnitude higher than the DMS and DMDS overall average emissions rates, determined as 0.017 g day(-1) AU(-1) and 0.036 g day(-1) AU(-1), respectively. The overall average lagoon flux was 1.33 mu g m(-2) min(-1) for H2S, which was approximately an order of magnitude higher than the overall average DMS (0.12 mu g m(-2) min(-1)) and DMDS (0.09 mu g m(-2) min(-1)) lagoon fluxes. The overall average lagoon emission for H2S (0.038 g day(-1) AU(-1)) was also approximately an order of magnitude higher than the overall average DMS (0.0034 g day(-1) AU(-1)) and DMDS (0.0028 g day(-1) AU(-1)) emissions. H2S, DMS and DMDS have offensive odors and low odor thresholds. Over all four sampling seasons, 77% of 15 min averaged H2S barn concentrations were an order of magnitude above the average odor threshold. During these sampling periods, however, DMS and DMDS concentrations did not exceed their odor thresholds. The overall average barn and lagoon emissions from this study were used to help estimate barn, lagoon and total (barn + lagoon) RSC emissions from swine CAFOs in North Carolina. Total (barn + lagoon) H2S emissions from swine CAFOs in North Carolina were estimated to be 1.22*10(6) kg yr(-1). The barns had significantly higher H2S emissions than the lagoons, contributing approximate to 98% of total North Carolina H2S swine CAFO emissions. Total (barn + lagoon) emissions for DMS and DMDS were 1-2 orders of magnitude lower, with barns contributing approximate to 86% and approximate to 93% of total emissions, respectively. H2S swine CAFO emissions were estimated to contribute approximate to 18% of North Carolina H2S emissions. (C) 2014 Elsevier Ltd. All rights reserved. |
英文关键词 | Reduced sulfur compounds;Hydrogen sulfide;CAFO emissions;Swine |
语种 | 英语 |
WOS记录号 | WOS:000340316300050 |
来源期刊 | ATMOSPHERIC ENVIRONMENT
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来源机构 | 美国环保署 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/58230 |
作者单位 | 1.N Carolina State Univ, Dept Marine Earth & Atmospher Sci, Raleigh, NC 27695 USA; 2.US EPA, Sr Environm Employment Program, Res Triangle Pk, NC 27711 USA |
推荐引用方式 GB/T 7714 | Rumsey, Ian C.,Aneja, Viney P.,Lonneman, William A.. Characterizing reduced sulfur compounds emissions from a swine concentrated animal feeding operation[J]. 美国环保署,2014,94:458-466. |
APA | Rumsey, Ian C.,Aneja, Viney P.,&Lonneman, William A..(2014).Characterizing reduced sulfur compounds emissions from a swine concentrated animal feeding operation.ATMOSPHERIC ENVIRONMENT,94,458-466. |
MLA | Rumsey, Ian C.,et al."Characterizing reduced sulfur compounds emissions from a swine concentrated animal feeding operation".ATMOSPHERIC ENVIRONMENT 94(2014):458-466. |
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