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DOI10.1080/02786826.2017.1423174
Continuous flow hygroscopicity-resolved relaxed eddy accumulation (Hy-Res REA) method of measuring size-resolved sodium chloride particle fluxes
Meskhidze, N.1; Royalty, T. M.1; Phillips, B. N.1; Dawson, K. W.1; Petters, M. D.1; Reed, R.2; Weinstein, J. P.3; Hook, D. A.3; Wiener, R. W.3
发表日期2018
ISSN0278-6826
卷号52期号:4页码:433-450
英文摘要

The accurate representation of aerosols in climate models requires direct ambient measurement of the size- and composition-dependent particle production fluxes. Here, we present the design, testing, and analysis of data collected through the first instrument capable of measuring hygroscopicity-based, size-resolved particle fluxes using a continuous-flow Hygroscopicity-Resolved Relaxed Eddy Accumulation (Hy-Res REA) technique. The Hy-Res REA system used in this study includes a 3D sonic anemometer, two fast-response solenoid valves, two condensation particle counters, a scanning mobility particle sizer, and a hygroscopicity tandem differential mobility analyzer. The different components of the instrument were tested inside the US Environmental Protection Agency's Aerosol Test Facility for sodium chloride and ammonium sulfate particle fluxes. The new REA system design does not require particle accumulation, and therefore avoids the diffusional wall losses associated with long residence times of particles inside the air collectors of traditional REA devices. A linear relationship was found between the sodium chloride particle fluxes measured by eddy covariance and REA techniques. The particle detection limit of the Hy-Res REA flux system is estimated to be approximate to 3 x 10(5) m(-2) s(-1). The estimated sodium chloride particle classification limit, for the mixture of sodium chloride and ammonium sulfate particles of comparable concentrations, is approximate to 6 x 10(6) m(-2) s(-1).Copyright (c) 2018 American Association for Aerosol Research


语种英语
WOS记录号WOS:000428191600001
来源期刊AEROSOL SCIENCE AND TECHNOLOGY
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/58184
作者单位1.North Carolina State Univ, Dept Marine Earth & Atmospher Sci, Campus Box 8208, Raleigh, NC 27695 USA;
2.North Carolina State Univ, Dept Appl Ecol, Raleigh, NC USA;
3.US EPA, Natl Exposure Res Lab, Res Triangle Pk, NC 27711 USA
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Meskhidze, N.,Royalty, T. M.,Phillips, B. N.,et al. Continuous flow hygroscopicity-resolved relaxed eddy accumulation (Hy-Res REA) method of measuring size-resolved sodium chloride particle fluxes[J]. 美国环保署,2018,52(4):433-450.
APA Meskhidze, N..,Royalty, T. M..,Phillips, B. N..,Dawson, K. W..,Petters, M. D..,...&Wiener, R. W..(2018).Continuous flow hygroscopicity-resolved relaxed eddy accumulation (Hy-Res REA) method of measuring size-resolved sodium chloride particle fluxes.AEROSOL SCIENCE AND TECHNOLOGY,52(4),433-450.
MLA Meskhidze, N.,et al."Continuous flow hygroscopicity-resolved relaxed eddy accumulation (Hy-Res REA) method of measuring size-resolved sodium chloride particle fluxes".AEROSOL SCIENCE AND TECHNOLOGY 52.4(2018):433-450.
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