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DOI | 10.1080/02786826.2017.1423174 |
Continuous flow hygroscopicity-resolved relaxed eddy accumulation (Hy-Res REA) method of measuring size-resolved sodium chloride particle fluxes | |
Meskhidze, N.1; Royalty, T. M.1; Phillips, B. N.1; Dawson, K. W.1; Petters, M. D.1; Reed, R.2; Weinstein, J. P.3; Hook, D. A.3; Wiener, R. W.3 | |
发表日期 | 2018 |
ISSN | 0278-6826 |
卷号 | 52期号:4页码:433-450 |
英文摘要 | The accurate representation of aerosols in climate models requires direct ambient measurement of the size- and composition-dependent particle production fluxes. Here, we present the design, testing, and analysis of data collected through the first instrument capable of measuring hygroscopicity-based, size-resolved particle fluxes using a continuous-flow Hygroscopicity-Resolved Relaxed Eddy Accumulation (Hy-Res REA) technique. The Hy-Res REA system used in this study includes a 3D sonic anemometer, two fast-response solenoid valves, two condensation particle counters, a scanning mobility particle sizer, and a hygroscopicity tandem differential mobility analyzer. The different components of the instrument were tested inside the US Environmental Protection Agency's Aerosol Test Facility for sodium chloride and ammonium sulfate particle fluxes. The new REA system design does not require particle accumulation, and therefore avoids the diffusional wall losses associated with long residence times of particles inside the air collectors of traditional REA devices. A linear relationship was found between the sodium chloride particle fluxes measured by eddy covariance and REA techniques. The particle detection limit of the Hy-Res REA flux system is estimated to be approximate to 3 x 10(5) m(-2) s(-1). The estimated sodium chloride particle classification limit, for the mixture of sodium chloride and ammonium sulfate particles of comparable concentrations, is approximate to 6 x 10(6) m(-2) s(-1).Copyright (c) 2018 American Association for Aerosol Research |
语种 | 英语 |
WOS记录号 | WOS:000428191600001 |
来源期刊 | AEROSOL SCIENCE AND TECHNOLOGY
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来源机构 | 美国环保署 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/58184 |
作者单位 | 1.North Carolina State Univ, Dept Marine Earth & Atmospher Sci, Campus Box 8208, Raleigh, NC 27695 USA; 2.North Carolina State Univ, Dept Appl Ecol, Raleigh, NC USA; 3.US EPA, Natl Exposure Res Lab, Res Triangle Pk, NC 27711 USA |
推荐引用方式 GB/T 7714 | Meskhidze, N.,Royalty, T. M.,Phillips, B. N.,et al. Continuous flow hygroscopicity-resolved relaxed eddy accumulation (Hy-Res REA) method of measuring size-resolved sodium chloride particle fluxes[J]. 美国环保署,2018,52(4):433-450. |
APA | Meskhidze, N..,Royalty, T. M..,Phillips, B. N..,Dawson, K. W..,Petters, M. D..,...&Wiener, R. W..(2018).Continuous flow hygroscopicity-resolved relaxed eddy accumulation (Hy-Res REA) method of measuring size-resolved sodium chloride particle fluxes.AEROSOL SCIENCE AND TECHNOLOGY,52(4),433-450. |
MLA | Meskhidze, N.,et al."Continuous flow hygroscopicity-resolved relaxed eddy accumulation (Hy-Res REA) method of measuring size-resolved sodium chloride particle fluxes".AEROSOL SCIENCE AND TECHNOLOGY 52.4(2018):433-450. |
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