气候变化领域集成服务门户(CCPortal): Impact of iron-modified biochars on soil nitrous oxide emissions: Variations with iron salts and soil fertility

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DOI	10.1016/j.jenvman.2024.120571
	Impact of iron-modified biochars on soil nitrous oxide emissions: Variations with iron salts and soil fertility
	Liao, Xiaolin; Mao, Shuxia; Shan, Yongxin; Gao, Wenran; Wang, Shengsen; Malghani, Saadatullah
发表日期	2024
ISSN	0301-4797
EISSN	1095-8630
起始页码	356
卷号	356
英文摘要	Nitrous oxide (N2O) emissions from soils are a significant environmental concern due to their contribution to greenhouse gas emissions. Biochar has been considered as a promising soil amendment for its potential to influence soil processes. Iron modification of biochar has been extensively discussed for its ability to enhance adsorption of pollutants, yet its impact on mitigating soil N2O emissions remains poorly understood. In the present study, corn straw (CB) and wood (WB) biochars were treated with FeSO4/FeCl3 (SCB and SWB) and Fe (NO3)(3) (NCB and NWB). The effects of these biochars on soil N2O emissions were investigated using soils with varying fertility levels over a 35-day incubation period at 20 degrees C. Results revealed significant variations in biochar surface chemistry depending on biochar feedstock and iron salts. Compared to pristine biochars, NWB and NCB exhibited higher pH, total N content, and dissolved NO3-N concentrations (246 +/- 17 and 298 +/- 35 mg kg(-1), respectively), but lower bulk and surface C content. In contrast, SWB and SCB demonstrated acidic pH and elevated dissolved NH4-N concentrations (5.38 +/- 0.43 and 4.19 +/- 0.22 mg kg(-1), respectively). In forest soils, NWB and NCB increased cumulative N2O emission by 28.5% and 67.0%, respectively, likely due to the introduction of mineral nitrogen evidenced by significant positive correlation with NO3-N or NH4-N. Conversely, SWB and SCB reduced emissions in the same soil by 28.5% and 6.9%, respectively. In agricultural soil, most biochars, except SWB, enhanced N2O emissions, possibly through the release of labile organic carbon facilitating denitrification. These findings underscore the significance of changes in biochar surface chemistry and the associated potential risk in triggering soil N2O emissions. This study highlights the need for a balanced design of biochar that considers both engineering benefits and climate change mitigation.
英文关键词	Biochar surface chemistry; Nitrification; Denitrification; Functional genes
语种	英语
WOS研究方向	Environmental Sciences & Ecology
WOS类目	Environmental Sciences
WOS记录号	WOS:001221171300001
来源期刊	JOURNAL OF ENVIRONMENTAL MANAGEMENT
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/301866
作者单位	Nanjing Forestry University; Nanjing Forestry University; Yangzhou University; University of Copenhagen
推荐引用方式 GB/T 7714	Liao, Xiaolin,Mao, Shuxia,Shan, Yongxin,et al. Impact of iron-modified biochars on soil nitrous oxide emissions: Variations with iron salts and soil fertility[J],2024,356.
APA	Liao, Xiaolin,Mao, Shuxia,Shan, Yongxin,Gao, Wenran,Wang, Shengsen,&Malghani, Saadatullah.(2024).Impact of iron-modified biochars on soil nitrous oxide emissions: Variations with iron salts and soil fertility.JOURNAL OF ENVIRONMENTAL MANAGEMENT,356.
MLA	Liao, Xiaolin,et al."Impact of iron-modified biochars on soil nitrous oxide emissions: Variations with iron salts and soil fertility".JOURNAL OF ENVIRONMENTAL MANAGEMENT 356(2024).