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DOI10.1021/acs.est.4c02826
Glucose Enhances Salinity-Driven Sea Spray Aerosol Production in Eastern Arctic Waters
发表日期2024
ISSN0013-936X
EISSN1520-5851
起始页码58
结束页码20
卷号58期号:20
英文摘要Sea spray aerosols (SSA) greatly affect the climate system by scattering solar radiation and acting as seeds for cloud droplet formation. The ecosystems in the Arctic Ocean are rapidly changing due to global warming, and the effects these changes have on the generation of SSA, and thereby clouds and fog formation in this region, are unknown. During the ship-based Arctic Century Expedition, we examined the dependency of forced SSA production on the biogeochemical characteristics of seawater using an on-board temperature-controlled aerosol generation chamber with a plunging jet system. Our results indicate that mainly seawater salinity and organic content influence the production and size distribution of SSA. However, we observed a 2-fold higher SSA production from waters with similar salinity collected north of 81 degrees N compared to samples collected south of this latitude. This variability was not explained by phytoplankton and bacterial abundances or Chlorophyll-a concentration but by the presence of glucose in seawater. The synergic action of sea salt (essential component) and glucose or glucose-rich saccharides (enhancer) accounts for >80% of SSA predictability throughout the cruise. Our results suggest that besides wind speed and salinity, SSA production in Arctic waters is also affected by specific organics released by the microbiota.
英文关键词marine biogeochemistry; Arctic; polar aerosolproduction; aerosol chamber; organic matter; climate change
语种英语
WOS研究方向Engineering ; Environmental Sciences & Ecology
WOS类目Engineering, Environmental ; Environmental Sciences
WOS记录号WOS:001225082300001
来源期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/296192
作者单位Consejo Superior de Investigaciones Cientificas (CSIC); CSIC - Centro Mediterraneo de Investigaciones Marinas y Ambientales (CMIMA); CSIC - Instituto de Ciencias del Mar (ICM); University of Barcelona; Helmholtz Association; GEOMAR Helmholtz Center for Ocean Research Kiel; Finnish Meteorological Institute; Swiss Federal Institutes of Technology Domain; ETH Zurich; Arctic & Antarctic Research Institute; Swiss Federal Institutes of Technology Domain; Ecole Polytechnique Federale de Lausanne
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. Glucose Enhances Salinity-Driven Sea Spray Aerosol Production in Eastern Arctic Waters[J],2024,58(20).
APA (2024).Glucose Enhances Salinity-Driven Sea Spray Aerosol Production in Eastern Arctic Waters.ENVIRONMENTAL SCIENCE & TECHNOLOGY,58(20).
MLA "Glucose Enhances Salinity-Driven Sea Spray Aerosol Production in Eastern Arctic Waters".ENVIRONMENTAL SCIENCE & TECHNOLOGY 58.20(2024).
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