气候变化领域集成服务门户(CCPortal): Boosting CO2 piezo-reduction via metal-support interactions in Au/ZnO based catalysts

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DOI	10.1016/j.jcis.2024.01.169
	Boosting CO2 piezo-reduction via metal-support interactions in Au/ZnO based catalysts
	Zhou, Rundong; Wu, Di; Ma, Jiangping; Ruan, Lujie; Feng, Yajie; Ban, Chaogang; Zhou, Kai; Cai, Songjiang; Gan, Li -Yong; Zhou, Xiaoyuan
发表日期	2024
ISSN	0021-9797
EISSN	1095-7103
起始页码	661
卷号	661
英文摘要	Confronting the challenge of climate change necessitates innovative approaches for the reduction of CO2 emissions. Metal -support interaction has been widely demonstrated to enable greatly improved performances in thermal -catalytic, photocatalytic and electrocatalytic CO2 reduction. However, its applicability and specifically its role in the emerging piezo-electrocatalytic CO2 reduction are unknown, severely hampering the utilizations of piezo-electrocatalysis in CO2 conversion. Herein, by adopting Au particles supported on ZnO (Au/ZnO) as a paradigm, it is found that the metal -support interaction can remarkably improve the separation and transfer of piezo-carriers and enhance CO2 adsorption. As a result, Au/ZnO demonstrates a substantially boosted activity for piezo-electrocatalytic CO2 reduction and the optimal sample exhibits a 37.3% increase in CO yield compared to the pristine ZnO. The integration of metal -support interactions opens a new avenue to the design of advanced piezo-electrocatalysts for CO2 reduction.
英文关键词	Metal -support interaction; Au/ZnO; Piezo-electrocatalysis; CO 2 reduction
语种	英语
WOS研究方向	Chemistry
WOS类目	Chemistry, Physical
WOS记录号	WOS:001176217800001
来源期刊	JOURNAL OF COLLOID AND INTERFACE SCIENCE
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/291849
作者单位	University of Cambridge; Chongqing University; Chongqing University; Chongqing University
推荐引用方式 GB/T 7714	Zhou, Rundong,Wu, Di,Ma, Jiangping,et al. Boosting CO2 piezo-reduction via metal-support interactions in Au/ZnO based catalysts[J],2024,661.
APA	Zhou, Rundong.,Wu, Di.,Ma, Jiangping.,Ruan, Lujie.,Feng, Yajie.,...&Zhou, Xiaoyuan.(2024).Boosting CO2 piezo-reduction via metal-support interactions in Au/ZnO based catalysts.JOURNAL OF COLLOID AND INTERFACE SCIENCE,661.
MLA	Zhou, Rundong,et al."Boosting CO2 piezo-reduction via metal-support interactions in Au/ZnO based catalysts".JOURNAL OF COLLOID AND INTERFACE SCIENCE 661(2024).