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DOI10.1038/s41561-022-00921-6
Fluocerite as a precursor to rare earth element fractionation in ore-forming systems
Strzelecki A.C.;   Migdisov A.;   Boukhalfa H.;   Sauer K.;   McIntosh K.G.;   Currier R.P.;   Williams-Jones A.E.;   Guo X.
发表日期2022
ISSN1752-0894
起始页码327
结束页码333
卷号15期号:4
英文摘要Emerging renewable energy technologies and low-carbon transportation rely heavily on the unique optical and magnetic properties of the rare earth elements. The medium to heavy rare earth elements, neodymium to lutetium, are most sought by industry but are the least abundant in nature. Only a small proportion of known rare earth element deposits are enriched in these elements. Identifying additional sources of medium to heavy rare earth elements for resource exploration requires improved understanding of the mechanisms responsible for the formation of such highly fractionated deposits. Here we report the results of experiments demonstrating a mechanism that could lead to enrichment of medium to heavy rare earth elements in ore-forming hydrothermal systems. In our experiments, we simulated natural hydrothermal systems by heating a column containing apatite and fluorite through which we pumped a chloride-rich solution bearing rare earth elements. Analysis of our experiments shows that the fluoride mineral fluocerite can serve as a precursor phase that fractionates rare earth elements before it is subsequently converted to a thermodynamically more stable mineral. Our findings identify geological settings in which fluocerite is observed or predicted to occur as potential exploration targets for deposits enriched in medium to heavy rare earth elements. © 2022, The Author(s), under exclusive licence to Springer Nature Limited.
语种英语
scopus关键词alternative energy; apatite; exploration; fluorite; fractionation; heating; neodymium; rare earth element; thermodynamic property; thermodynamics
来源期刊Nature Geoscience
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/262217
作者单位Los Alamos National Laboratory, Earth and Environmental Sciences Division, Los Alamos, NM, United States
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Strzelecki A.C.; Migdisov A.; Boukhalfa H.; Sauer K.; McIntosh K.G.; Currier R.P.; Williams-Jones A.E.; Guo X.. Fluocerite as a precursor to rare earth element fractionation in ore-forming systems[J],2022,15(4).
APA Strzelecki A.C.; Migdisov A.; Boukhalfa H.; Sauer K.; McIntosh K.G.; Currier R.P.; Williams-Jones A.E.; Guo X..(2022).Fluocerite as a precursor to rare earth element fractionation in ore-forming systems.Nature Geoscience,15(4).
MLA Strzelecki A.C.; Migdisov A.; Boukhalfa H.; Sauer K.; McIntosh K.G.; Currier R.P.; Williams-Jones A.E.; Guo X.."Fluocerite as a precursor to rare earth element fractionation in ore-forming systems".Nature Geoscience 15.4(2022).
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