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DOI10.1016/j.envpol.2020.115272
New insights into particle-bound trace elements in surface snow, Eastern Tien Shan, China
Huang, Ju; Wu, Guangjian; Zhang, Xuelei; Zhang, Chenglong
通讯作者Wu, GJ (通讯作者)
发表日期2020
ISSN0269-7491
EISSN1873-6424
卷号267
英文摘要Trace elements (TEs) in the insoluble particles of surface snow are less affected by melting processes and can be used as environmental proxies to reveal natural and anthropogenic emissions. Here the first comprehensive study of the 16 TEs (Al, As, Ba, Bi, Cr, Cu, Fe, Mn, Ni, Pb, Sn, Sr, Ti, U, V, and Zn) in insoluble particles (>0.45 mm) from surface snow samples collected at Urumqi Glacier No. 1 (UG1), Eastern Tien Shan, China, from February 2008 to January 2010 were presented. Results show that concentrations of most insoluble particulate TEs (TEs insol) in the snow were higher in summer while lower in winter, due to the increasing particle inputs and melting processes. The abundances of As, Cr, Cu, Ni, Pb, and Zn in some samples were higher than those in surrounding urban soils, which might due to these TEs have further anthropogenic input beyond the already contaminated re-suspended urban soil particles and TEs were mainly enriched in particles with small grain size. Based on enrichment factor (EF) and principal component analysis (PCA), our results suggest that eight TEs (Al, Fe, Ti, Ba, Mn, Sr, U, and V) mainly came from mineral dust, while the remaining eight TEs (As, Bi, Cr, Cu, Ni, Pb, Sn, and Zn) were affected by coal combustion, mining and smelting of non-ferrous metals, traffic emissions, and the steel industry. The Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model suggests that pollutants might originate from Xinjiang province, Kazakhstan, and Kyrgyzstan. Moreover, UG1 received more significant inputs of particle-bound pollutants in summer than in winter due to the stronger convection and the prevailing valley wind that transports pollutants from the city of Urumqi. (C) 2020 Elsevier Ltd. All rights reserved.
关键词CONTAMINATIONINDUSTRIALEMISSIONSREGIONSFLUXESMETALSLEAD
英文关键词Elemental composition; Seasonal variation; Pollution assessment; Sources; Glacier
语种英语
WOS研究方向Environmental Sciences & Ecology
WOS类目Environmental Sciences
WOS记录号WOS:000593965600020
来源期刊ENVIRONMENTAL POLLUTION
来源机构中国科学院青藏高原研究所
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/259867
推荐引用方式
GB/T 7714
Huang, Ju,Wu, Guangjian,Zhang, Xuelei,et al. New insights into particle-bound trace elements in surface snow, Eastern Tien Shan, China[J]. 中国科学院青藏高原研究所,2020,267.
APA Huang, Ju,Wu, Guangjian,Zhang, Xuelei,&Zhang, Chenglong.(2020).New insights into particle-bound trace elements in surface snow, Eastern Tien Shan, China.ENVIRONMENTAL POLLUTION,267.
MLA Huang, Ju,et al."New insights into particle-bound trace elements in surface snow, Eastern Tien Shan, China".ENVIRONMENTAL POLLUTION 267(2020).
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