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DOI | 10.1016/j.chemosphere.2020.125843 |
High particulate carbon deposition in Lhasad-a typical city in the Himalayan-Tibetan Plateau due to local contributions | |
Yan, Fangping; Wang, Pengling; Kang, Shichang; Chen, Pengfei; Hu, Zhaofu; Han, Xiaowen; Sillanpaa, Mika; Li, Chaoliu | |
通讯作者 | Li, CL (通讯作者) |
发表日期 | 2020 |
ISSN | 0045-6535 |
EISSN | 1879-1298 |
卷号 | 247 |
英文摘要 | The Himalayan-Tibetan Plateau is a typical remote region with sparse air pollution. However, air pollution in cites of the inner Himalayan-Tibetan Plateau is relatively serious due to emissions from local residents. Carbonaceous aerosols are not only an important component of air pollutants that affect the health of local residents but also an important trigger of climate change. In this study, the annual wet and dry deposition rates of carbonaceous particles were investigated in Lhasad-a typical city in the Himalayan-Tibetan Plateau, by collecting precipitation and dry deposition samples and analyzing with a thermal-optical measurement protocol. The results showed that the in-situ annual wet deposition rates of water-insoluble organic carbon (WIOC) and black carbon (BC) were 169.6 and 19.4 mg m(-2) yr(-1), respectively, with the highest and lowest values occurring in the monsoon and non-monsoon periods, respectively. Both precipitation amounts and concentrations of WIOC and BC contributed to wet deposition rates. The dry deposition rates of WIOC and BC in Lhasa had an opposite seasonal variation to that of wet deposition, with annual average deposition rates of 2563.9 and 165.7 mg m(-2) yr(-1), respectively, which were much higher than those of the nearby glacier region and remote area. These values were also much higher than the results from modeling and empirical calculations, indicating that Lhasa is a high pollution point that cannot capture by models. The results in this study have significant implications for the transport of local emissions in Lhasa to the nearby remote and glacier regions. (C) 2020 Elsevier Ltd. All rights reserved. |
关键词 | LIGHT-ABSORPTION CHARACTERISTICSDISSOLVED ORGANIC-CARBONTHERMAL/OPTICAL REFLECTANCE METHOD3 REMOTE STATIONSBLACK CARBONWET DEPOSITIONATMOSPHERIC DEPOSITIONELEMENTAL CARBONISOTOPIC COMPOSITIONCHEMICAL-COMPOSITION |
英文关键词 | Black carbon; Organic carbon; Lhasa; Dry and wet deposition |
语种 | 英语 |
WOS研究方向 | Environmental Sciences & Ecology |
WOS类目 | Environmental Sciences |
WOS记录号 | WOS:000527924400038 |
来源期刊 | CHEMOSPHERE
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来源机构 | 中国科学院青藏高原研究所 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/259846 |
推荐引用方式 GB/T 7714 | Yan, Fangping,Wang, Pengling,Kang, Shichang,et al. High particulate carbon deposition in Lhasad-a typical city in the Himalayan-Tibetan Plateau due to local contributions[J]. 中国科学院青藏高原研究所,2020,247. |
APA | Yan, Fangping.,Wang, Pengling.,Kang, Shichang.,Chen, Pengfei.,Hu, Zhaofu.,...&Li, Chaoliu.(2020).High particulate carbon deposition in Lhasad-a typical city in the Himalayan-Tibetan Plateau due to local contributions.CHEMOSPHERE,247. |
MLA | Yan, Fangping,et al."High particulate carbon deposition in Lhasad-a typical city in the Himalayan-Tibetan Plateau due to local contributions".CHEMOSPHERE 247(2020). |
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