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DOI10.1016/j.cej.2021.131958
Study of the sorption/desorption behavior of chlortetracycline on sediments in the upper reaches of the Yellow River
Liang, Xinru; Liu, Lanlan; Jiang, Yufeng; Nan, Zhijiang; Deng, Xueru; Ma, Fengfeng; Wang, Gang; Wu, Yingqin
通讯作者Jiang, YF (通讯作者),Lanzhou Jiaotong Univ, Sch Environm & Municipal Engn, Lanzhou 730070, Peoples R China.
发表日期2022
ISSN1385-8947
EISSN1873-3212
卷号428
英文摘要The presence of antibiotic in aquatic environments has become a topic of great concern with respect to both environment and global public health. However, to date, only a few studies have been carried out on the sorption behavior of antibiotics in aquatic environments. In this study, batch equilibrium experiments were conducted to explore the sorption/desorption behavior of Chlortetracycline (CTC) on the sediments in the Lanzhou section of the Yellow River. The results showed multilayer chemisorption on heterogeneous surfaces dominated by hydrophobic distribution and an obvious hysteresis phenomenon was observed. In addition, the sorption was found to be influenced by factors such as a continuous increase in the temperature, reduction in the initial concentration of CTC, and the increasing particle size of the sediments. The pH was found to affect the dissociation degree of CTC, and the sorptive amount was found to decrease with the increase in the pH value. The presence of other ions which with high valence state and concentration presenting an obvious inhibitory effect in the sorption process. Additionally, the large sorptive amount of antibiotics in the sediments due to the high Cation exchange capacity (CEC), organic matter, and clay particles indicated the influence of the physicochemical properties of sediments on the sorption behavior of antibiotics. This study preliminarily grasps the trend of CTC sorption/desorption on sediments, which is helpful in understanding the fate of CTC and assessing its ecological risks in the upper reaches of the Yellow River.
关键词AQUEOUS-SOLUTIONSULFONAMIDE ANTIBIOTICSVETERINARY DRUGSSURFACE-WATERSORPTIONADSORPTIONSOILSKINETICSOXYTETRACYCLINEDYE
英文关键词Sorption; desorption; Influential factors; Chlortetracycline; Sediment; Yellow River
语种英语
WOS研究方向Engineering
WOS类目Engineering, Environmental ; Engineering, Chemical
WOS记录号WOS:000728388500008
来源期刊CHEMICAL ENGINEERING JOURNAL
来源机构中国科学院西北生态环境资源研究院
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/254884
作者单位[Liang, Xinru; Liu, Lanlan; Jiang, Yufeng; Nan, Zhijiang; Deng, Xueru; Ma, Fengfeng; Wang, Gang] Lanzhou Jiaotong Univ, Sch Environm & Municipal Engn, Lanzhou 730070, Peoples R China; [Liang, Xinru; Jiang, Yufeng; Nan, Zhijiang; Deng, Xueru; Ma, Fengfeng; Wang, Gang] Lanzhou Jiaotong Univ, Key Lab Yellow River Water Environm Gansu Prov, Lanzhou 730070, Peoples R China; [Wu, Yingqin] Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, Key Lab Petr Resources Res, Lanzhou 730000, Peoples R China
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Liang, Xinru,Liu, Lanlan,Jiang, Yufeng,et al. Study of the sorption/desorption behavior of chlortetracycline on sediments in the upper reaches of the Yellow River[J]. 中国科学院西北生态环境资源研究院,2022,428.
APA Liang, Xinru.,Liu, Lanlan.,Jiang, Yufeng.,Nan, Zhijiang.,Deng, Xueru.,...&Wu, Yingqin.(2022).Study of the sorption/desorption behavior of chlortetracycline on sediments in the upper reaches of the Yellow River.CHEMICAL ENGINEERING JOURNAL,428.
MLA Liang, Xinru,et al."Study of the sorption/desorption behavior of chlortetracycline on sediments in the upper reaches of the Yellow River".CHEMICAL ENGINEERING JOURNAL 428(2022).
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