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DOI | 10.1016/j.colsurfa.2022.128574 |
Solar-driven photothermal-Fenton removal of ofloxacin through waste natural pyrite with dual-function | |
Zhang, Qian; Zheng, Dan; Bai, Bo; Hu, Na; Wang, Honglun | |
通讯作者 | Bai, B (通讯作者),Changan Univ, Key Lab Subsurface Hydrol & Ecol Effects Arid Reg, Minist Educ, Xian 710054, Peoples R China. |
发表日期 | 2022 |
ISSN | 0927-7757 |
EISSN | 1873-4359 |
卷号 | 641 |
英文摘要 | The solar-driven photothermal-Fenton catalytic is demonstrated to be a promising technology to remove pollutants from wastewater benefiting from their low cost and high removal efficiency. Here, we constructed a photothermal-Fenton system using waste natural pyrite as dual-function material with Fenton catalytic and photothermal functions for the first time to remove ofloxacin. The removal efficiency was up to 94.7% and the removal rate was 6.85 times higher than that in conventional Fenton reaction, which was attributed to the synergistic interaction of the photothermal conversion and the Fenton of pyrite. The quenching experiments demonstrated & BULL;OH and h(+) were the dominantly active free radicals. The pyrite had performed substantial removal efficiency during a wide pH range (3-9) and exhibited excellent stability after six cycles. Besides, the continuous flow experiment under natural solar irradiation was also conducted to evaluate the ability of actual application. The research realizes the full utilization of waste pyrite and provides new avenues for the application of solar-driven photothermal effect in environmental remediation. |
关键词 | NANOPARTICLESDEGRADATIONRESONANCECATALYSTSSURFACE |
英文关键词 | Pyrite; Photothermal conversion; Fenton; Waste utilization; Ofloxacin |
语种 | 英语 |
WOS研究方向 | Chemistry |
WOS类目 | Chemistry, Physical |
WOS记录号 | WOS:000772832000004 |
来源期刊 | COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
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来源机构 | 中国科学院西北生态环境资源研究院 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/254353 |
作者单位 | [Zhang, Qian; Zheng, Dan; Bai, Bo] Changan Univ, Key Lab Subsurface Hydrol & Ecol Effects Arid Reg, Minist Educ, Xian 710054, Peoples R China; [Zhang, Qian; Zheng, Dan; Bai, Bo] Changan Univ, Sch Water & Environm, Xi'an 710054, Peoples R China; [Bai, Bo; Hu, Na; Wang, Honglun] Chinese Acad Sci, Northwest Inst Plateau Biol, Key Lab Tibetan Med Res, Xining 810008, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Qian,Zheng, Dan,Bai, Bo,et al. Solar-driven photothermal-Fenton removal of ofloxacin through waste natural pyrite with dual-function[J]. 中国科学院西北生态环境资源研究院,2022,641. |
APA | Zhang, Qian,Zheng, Dan,Bai, Bo,Hu, Na,&Wang, Honglun.(2022).Solar-driven photothermal-Fenton removal of ofloxacin through waste natural pyrite with dual-function.COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,641. |
MLA | Zhang, Qian,et al."Solar-driven photothermal-Fenton removal of ofloxacin through waste natural pyrite with dual-function".COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 641(2022). |
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