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DOI	10.5194/acp-20-13579-2020
	Heterogeneous nucleation of water vapor on different types of black carbon particles
	Laaksonen A.; Malila J.; Nenes A.
发表日期	2020
ISSN	1680-7316
起始页码	13579
结束页码	13589
卷号	20 期号:21
英文摘要	The heterogeneous nucleation of water vapor on insoluble particles affects cloud formation, precipitation, the hydrological cycle, and climate. Despite its importance, heterogeneous nucleation remains a poorly understood phenomenon that relies heavily on empirical information for its quantitative description. Here, we examine the heterogeneous nucleation of water vapor on different types of soots as well as cloud drop activation of different types of soots, including both pure black carbon particles and black carbon particles mixed with secondary organic matter.We show that the recently developed adsorption nucleation theory quantitatively predicts the nucleation of water and droplet formation upon particles of the various soot types. A surprising consequence of this new understanding is that, with sufficient adsorption site density, soot particles can activate into cloud droplets - even when completely lacking any soluble material. © Author(s) 2020.
语种	英语
scopus关键词	adsorption; black carbon; cloud; nucleation; quantitative analysis; soot; water vapor
来源期刊	ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/247373
作者单位	Finnish Meteorological Institute, Helsinki, 00101, Finland; Department of Applied Physics, University of Eastern Finland, Kuopio, 70211, Finland; Nano and Molecular Systems Research Unit, University of Oulu, Oulu, 90014, Finland; Laboratory of Atmospheric Processes and their Impacts, School of Architecture, Civil and Environmental Engineering, École Polytechnique Federale de Lausanne, Lausanne, 1015, Switzerland; Institute of Chemical Engineering Sciences, Foundation for Research and Technology Hellas (FORTH/ICE-HT), Patras, 26504, Greece
推荐引用方式 GB/T 7714	Laaksonen A.,Malila J.,Nenes A.. Heterogeneous nucleation of water vapor on different types of black carbon particles[J],2020,20(21).
APA	Laaksonen A.,Malila J.,&Nenes A..(2020).Heterogeneous nucleation of water vapor on different types of black carbon particles.ATMOSPHERIC CHEMISTRY AND PHYSICS,20(21).
MLA	Laaksonen A.,et al."Heterogeneous nucleation of water vapor on different types of black carbon particles".ATMOSPHERIC CHEMISTRY AND PHYSICS 20.21(2020).