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DOI | 10.5194/acp-21-8677-2021 |
Substantial changes in gaseous pollutants and chemical compositions in fine particles in the North China Plain during the COVID-19 lockdown period: Anthropogenic vs. meteorological influences | |
Li R.; Zhao Y.; Fu H.; Chen J.; Peng M.; Wang C. | |
发表日期 | 2021 |
ISSN | 1680-7316 |
起始页码 | 8677 |
结束页码 | 8692 |
卷号 | 21期号:11 |
英文摘要 | The rapid response to the COVID-19 pandemic led to unprecedented decreases in economic activities, thereby reducing the pollutant emissions. A random forest (RF) model was applied to determine the respective contributions of meteorology and anthropogenic emissions to the changes in air quality. The result suggested that the strict lockdown measures significantly decreased primary components such as Cr (-67 %) and Fe (-61 %) in PM2:5 (p < 0:01), whereas the higher relative humidity (RH) and NH3 level and the lower air temperature (T) remarkably enhanced the production of secondary aerosol, including SO24-(29 %), NO-3 (29 %), and NHC 4 (21 %) (p < 0:05). The positive matrix factorization (PMF) result suggested that the contribution ratios of secondary formation (SF), industrial process (IP), biomass burning (BB), coal combustion (CC), and road dust (RD) changed from 36 %, 27 %, 21 %, 12 %, and 4 % before the COVID-19 outbreak to 44 %, 20 %, 20 %, 9 %, and 7 %, respectively. The rapid increase in the contribution ratio derived from SF to PM2:5 implied that the intermittent haze events during the COVID-19 period were characterized by secondary aerosol pollution, which was mainly contributed by the unfavorable meteorological conditions and high NH3 level. © 2021 Rui Li et al. |
语种 | 英语 |
scopus关键词 | aerosol; air quality; anthropogenic source; atmospheric pollution; chemical composition; chemical pollutant; COVID-19; disease control; emission inventory; pollution monitoring; China; North China Plain |
来源期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/246828 |
作者单位 | Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Institute of Atmospheric Sciences, Fudan University, Shanghai, 200433, China; Collaborative Innovation Center of Atmospheric Environment and Equipment Technology (CICAEET), Nanjing University of Information Science and Technology, Nanjing, 210044, China; School of Law of Tsinghua University, Beijing, 100084, China; Hebei Xianhe Environmental Protection Technology Co. Ltd, Shijiazhuang, 050035, China |
推荐引用方式 GB/T 7714 | Li R.,Zhao Y.,Fu H.,et al. Substantial changes in gaseous pollutants and chemical compositions in fine particles in the North China Plain during the COVID-19 lockdown period: Anthropogenic vs. meteorological influences[J],2021,21(11). |
APA | Li R.,Zhao Y.,Fu H.,Chen J.,Peng M.,&Wang C..(2021).Substantial changes in gaseous pollutants and chemical compositions in fine particles in the North China Plain during the COVID-19 lockdown period: Anthropogenic vs. meteorological influences.ATMOSPHERIC CHEMISTRY AND PHYSICS,21(11). |
MLA | Li R.,et al."Substantial changes in gaseous pollutants and chemical compositions in fine particles in the North China Plain during the COVID-19 lockdown period: Anthropogenic vs. meteorological influences".ATMOSPHERIC CHEMISTRY AND PHYSICS 21.11(2021). |
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