气候变化领域集成服务门户(CCPortal): Relating geostationary satellite measurements of aerosol optical depth (AOD) over East Asia to fine particulate matter (PM2.5): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model simulations

CCPortal

DOI	10.5194/acp-21-16775-2021
	Relating geostationary satellite measurements of aerosol optical depth (AOD) over East Asia to fine particulate matter (PM2.5): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model simulations
	Zhai S.; Jacob D.J.; Brewer J.F.; Li K.; Moch J.M.; Kim J.; Lee S.; Lim H.; Lee H.C.; Kuk S.K.; Park R.J.; Jeong J.I.; Wang X.; Liu P.; Luo G.; Yu F.; Meng J.; Martin R.V.; Travis K.R.; Hair J.W.; Anderson B.E.; Dibb J.E.; Jimenez J.L.; Campuzano-Jost P.; Nault B.A.; Woo J.-H.; Kim Y.; Zhang Q.; Liao H.
发表日期	2021
ISSN	1680-7316
起始页码	16775
结束页码	16791
卷号	21 期号:22
英文摘要	Geostationary satellite measurements of aerosol optical depth (AOD) over East Asia from the Geostationary Ocean Color Imager (GOCI) and Advanced Himawari Imager (AHI) instruments can augment surface monitoring of fine particulate matter (PM2.5) air quality, but this requires better understanding of the AOD-PM2.5 relationship. Here we use the GEOS-Chem chemical transport model to analyze the critical variables determining the AOD-PM2.5 relationship over East Asia by simulation of observations from satellite, aircraft, and ground-based datasets. This includes the detailed vertical aerosol profiling over South Korea from the KORUS-AQ aircraft campaign (May-June 2016) with concurrent ground-based PM2.5 composition, PM10, and AERONET AOD measurements. The KORUS-AQ data show that 550 nm AOD is mainly contributed by sulfate-nitrate-ammonium (SNA) and organic aerosols in the planetary boundary layer (PBL), despite large dust concentrations in the free troposphere, reflecting the optically effective size and high hygroscopicity of the PBL aerosols. We updated SNA and organic aerosol size distributions in GEOS-Chem to represent aerosol optical properties over East Asia by using in situ measurements of particle size distributions from KORUS-AQ. We find that SNA and organic aerosols over East Asia have larger size (number median radius of 0.11 μm with geometric standard deviation of 1.4) and 20 % larger mass extinction efficiency as compared to aerosols over North America (default setting in GEOS-Chem). Although GEOS-Chem is successful in reproducing the KORUS-AQ vertical profiles of aerosol mass, its ability to link AOD to PM2.5 is limited by under-accounting of coarse PM and by a large overestimate of nighttime PM2.5 nitrate. The GOCI-AHI AOD data over East Asia in different seasons show agreement with AERONET AODs and a spatial distribution consistent with surface PM2.5 network data. The AOD observations over North China show a summer maximum and winter minimum, opposite in phase to surface PM2.5. This is due to low PBL depths compounded by high residential coal emissions in winter and high relative humidity (RH) in summer. Seasonality of AOD and PM2.5 over South Korea is much weaker, reflecting weaker variation in PBL depth and lack of residential coal emissions. © 2021 Shixian Zhai et al.
语种	英语
scopus关键词	aerosol; airborne survey; computer simulation; EOS; geostationary satellite; ground-based measurement; numerical model; optical depth; particulate matter; Far East
来源期刊	ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/246434
作者单位	Harvard John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, United States; Department of Atmospheric Sciences, Yonsei University, Seoul, South Korea; Samsung Particulate Matter Research Institute, Samsung Advanced Institute of Technology, 130 Samsung-ro, Yeongtong-gu, Suwon-si, Gyeonggi-do, South Korea; School of Earth and Environmental Sciences, Seoul National University, Seoul, South Korea; School of Energy and Environment, City University of Hong Kong, Hong Kong, Hong Kong; School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA, United States; Atmospheric Sciences Research Center, University at Albany, Albany, NY, United States; Department of Atmospheric and Oceanic Sciences, University of California, Los Angeles, CA, United States; Department of Energy Environmental and Chemical Engineering, Washington University in St. Louis, St. Louis, MO, United States; NASA Langley Research Center, Hampton, VA, United States; Institute for ...
推荐引用方式 GB/T 7714	Zhai S.,Jacob D.J.,Brewer J.F.,et al. Relating geostationary satellite measurements of aerosol optical depth (AOD) over East Asia to fine particulate matter (PM2.5): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model simulations[J],2021,21(22).
APA	Zhai S..,Jacob D.J..,Brewer J.F..,Li K..,Moch J.M..,...&Liao H..(2021).Relating geostationary satellite measurements of aerosol optical depth (AOD) over East Asia to fine particulate matter (PM2.5): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model simulations.ATMOSPHERIC CHEMISTRY AND PHYSICS,21(22).
MLA	Zhai S.,et al."Relating geostationary satellite measurements of aerosol optical depth (AOD) over East Asia to fine particulate matter (PM2.5): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model simulations".ATMOSPHERIC CHEMISTRY AND PHYSICS 21.22(2021).