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DOI10.1029/2021JD034615
Isolating Large-Scale Smoke Impacts on Cloud and Precipitation Processes Over the Amazon With Convection Permitting Resolution
Herbert R.; Stier P.; Dagan G.
发表日期2021
ISSN2169-897X
卷号126期号:13
英文摘要Absorbing aerosol from biomass burning impacts the hydrological cycle and radiation fluxes both directly and indirectly via modifications to convective processes and cloud development. Using the ICOsahedral Non-hydrostatic modelling framework in a regional configuration with 1,500 m convection-permitting resolution, we isolate the response of the Amazonian atmosphere to biomass burning smoke via enhanced cloud droplet number concentrations Nd (aerosol-cloud interactions; ACI) and changes to radiative fluxes (aerosol-radiation interactions; ARI) over a period of 8 days. We decompose ARI into contributions from reduced shortwave radiation and localized heating of the smoke. We show ARI influences the formation and development of convective cells: surface cooling below the smoke drives suppression of convection that increases with smoke optical depth, while the elevated heating promotes initial suppression and subsequent intensification of convection overnight; a corresponding diurnal response (repeating temporal response day-after-day) from high precipitation rates is shown. Enhanced Nd (ACI) perturbs the bulk cloud properties and suppresses low-to-moderate precipitation rates. Both ACI and ARI result in enhanced high-altitude ice clouds that have a strong positive longwave radiative effect. Changes to low-cloud coverage (ARI) and albedo (ACI) drive an overall negative shortwave radiative effect, that slowly increases in magnitude due to a moistening of the boundary layer. The overall net radiative effect is dominated by the enhanced high-altitude clouds, and is sensitive to the plume longevity. The considerable diurnal responses that we simulate cannot be observed by polar orbiting satellites widely used in previous work, highlighting the potential of geostationary satellites to observe large-scale impacts of aerosols on clouds. © 2021. The Authors.
英文关键词aerosol-cloud interactions; Aerosol-radiation interactions; Amazon; biomass burning aerosol; cloud invigoration; high-resolution modeling
来源期刊Journal of Geophysical Research: Atmospheres
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/237138
作者单位Atmospheric, Oceanic and Planetary Physics, Department of Physics, University of Oxford, Oxford, United Kingdom
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Herbert R.,Stier P.,Dagan G.. Isolating Large-Scale Smoke Impacts on Cloud and Precipitation Processes Over the Amazon With Convection Permitting Resolution[J],2021,126(13).
APA Herbert R.,Stier P.,&Dagan G..(2021).Isolating Large-Scale Smoke Impacts on Cloud and Precipitation Processes Over the Amazon With Convection Permitting Resolution.Journal of Geophysical Research: Atmospheres,126(13).
MLA Herbert R.,et al."Isolating Large-Scale Smoke Impacts on Cloud and Precipitation Processes Over the Amazon With Convection Permitting Resolution".Journal of Geophysical Research: Atmospheres 126.13(2021).
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