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DOI10.1016/j.scib.2020.01.021
High loading cotton cellulose-based aerogel self-standing electrode for Li-S batteries
Mao H.; Liu L.; Shi L.; Wu H.; Lang J.; Wang K.; Zhu T.; Gao Y.; Sun Z.; Zhao J.; Gao G.; Zhang D.; Yan W.; Ding S.
发表日期2020
ISSN20959273
起始页码803
结束页码811
卷号65期号:10
英文摘要Lithium-sulfur (Li-S) batteries have attracted considerable attention due to their high energy density (2600 Wh kg−1). However, its commercialization is hindered seriously by the low loading and utilization rate of sulfur cathodes. Herein, we designed the cellulose-based graphene carbon composite aerogel (CCA) self-standing electrode to enhance the performance of Li-S batteries. The CCA contributes to the mass loading and utilization efficiency of sulfur, because of its unique physical structure: low density (0.018 g cm−3), large specific surface area (657.85 m2 g−1), high porosity (96%), and remarkable electrolyte adsorption (42.25 times). Compared to Al (about 49%), the CCA displayed excellent sulfur use efficiency (86%) and could reach to high area capacity of 8.60 mAh cm−2 with 9.11 mg S loading. Meanwhile, the CCA exhibits the excellent potential for pulse sensing applications due to its flexibility and superior sensitivity to electrical response signals. © 2020 Science China Press
关键词Cellulose-based graphene aerogelHigh sulfur loadingLithium-sulfur batteryPulse sensingSelf-standing electrode
英文关键词Aerogels; Carbon carbon composites; Cellulose; Electrodes; Electrolytes; Graphene; Lithium batteries; Lithium compounds; Graphene aerogels; High energy densities; Large specific surface areas; Pulse sensing; Self standings; Sensing applications; Sulfur loading; Utilization efficiency; Lithium sulfur batteries
语种英语
来源期刊Science Bulletin
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/207149
作者单位Xi'an Key Laboratory of Sustainable Energy Materials Chemistry, State Key Laboratory of Electrical Insulation and Power Equipment, Department of Applied Chemistry, School of Science, Xi'an Jiaotong University, Xi'an, 710049, China; Department of Environmental Science and Engineering, State Key Laboratory of Multiphase Flow in Power Engineering, Xi'an Jiaotong University, Xi'an, 710049, China
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Mao H.,Liu L.,Shi L.,et al. High loading cotton cellulose-based aerogel self-standing electrode for Li-S batteries[J],2020,65(10).
APA Mao H..,Liu L..,Shi L..,Wu H..,Lang J..,...&Ding S..(2020).High loading cotton cellulose-based aerogel self-standing electrode for Li-S batteries.Science Bulletin,65(10).
MLA Mao H.,et al."High loading cotton cellulose-based aerogel self-standing electrode for Li-S batteries".Science Bulletin 65.10(2020).
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