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DOI10.1039/d0ee03300f
Solar fuels and feedstocks: The quest for renewable black gold
Sayre H.J.; Tian L.; Son M.; Hart S.M.; Liu X.; Arias-Rotondo D.M.; Rand B.P.; Schlau-Cohen G.S.; Scholes G.D.
发表日期2021
ISSN17545692
起始页码1402
结束页码1419
卷号14期号:3
英文摘要Photocatalysis for organic synthesis is a tool capable of C-C, C-O and C-N bond transformations. This technology has the potential to transform the chemical manufacturing industry and support growing demand for chemical feedstocks. Compared to traditional catalysis, photocatalysis can access alternative reaction pathways that lower the overall energy requirement and operate at or near ambient conditions. A key challenge is the delivery of photoenergy at the scale required for rapid and efficient operation of the catalyst. The development of efficient, broad-spectrum light harvesting devices that funnel light energy to a catalyst, along with catalyst design to selectively enable high-energy reactions, are necessary steps towards solar fuels and feedstocks. This perspective highlights some recent advances in photocatalysis and advocates for expanding the scope of photocatalysis for large-scale industrial applications. © 2021 The Royal Society of Chemistry.
英文关键词Catalysts; Feedstocks; Gold; Light; Ambient conditions; Catalyst designs; Chemical feedstocks; Chemical manufacturing industries; Energy requirements; Light-harvesting; Organic synthesis; Reaction pathways; Photocatalysis; fuel; gold; renewable resource; solar power
语种英语
来源期刊Energy & Environmental Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/190737
作者单位Department of Chemistry, Princeton University, Princeton, NJ, United States; Department of Chemistry, University of Wisconsin-Madison, Madison, WI, United States; Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA, United States; Department of Electrical Engineering, Princeton University, Princeton, NJ, United States; Department of Chemistry, Kalamazoo College, Kalamazoo, MI, United States
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GB/T 7714
Sayre H.J.,Tian L.,Son M.,et al. Solar fuels and feedstocks: The quest for renewable black gold[J],2021,14(3).
APA Sayre H.J..,Tian L..,Son M..,Hart S.M..,Liu X..,...&Scholes G.D..(2021).Solar fuels and feedstocks: The quest for renewable black gold.Energy & Environmental Science,14(3).
MLA Sayre H.J.,et al."Solar fuels and feedstocks: The quest for renewable black gold".Energy & Environmental Science 14.3(2021).
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