气候变化领域集成服务门户(CCPortal): Biomimetic and bioinspired approaches for wiring enzymes to electrode interfaces

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DOI	10.1039/c6ee02801b
	Biomimetic and bioinspired approaches for wiring enzymes to electrode interfaces
	Saboe P.O.; Conte E.; Farell M.; Bazan G.C.; Kumar M.
发表日期	2017
ISSN	17545692
起始页码	14
结束页码	42
卷号	10 期号:1
英文摘要	Biomimetic and bioinspired approaches to redox enzyme wiring involve borrowing structures and strategies found in biological electron transfer systems for use in engineered devices. Redox protein-electrode systems are evolving for several applications, including energy, biomedical and environmental purposes. This review is intended to be both "tutorial" and comprehensive in that we provide a guide to understand, design, and improve electrode interfaces for redox enzyme electron transfer processes in devices. The review examines electrode interfaces by directly comparing them with biological electron transfer systems. First, the mechanisms, theory, and structures for electron transfer in biological systems are provided, followed by analysis of the strategies and structures engineered in redox-protein devices. The review describes the challenges of constructing and applying redox enzyme devices, including the poor electrical contact between electrodes and enzymes and low lifetime and scalability of devices. © The Royal Society of Chemistry 2017.
英文关键词	Biomimetics; Electrodes; Electron transitions; Enzymes; Bio-inspired approach; Electrical contacts; Electrode interface; Electrode systems; Electron transfer; Electron transfer process; Engineered devices; Redox proteins; Enzyme electrodes; design; electrode; electron; enzyme activity; protein; redox conditions
语种	英语
来源期刊	Energy & Environmental Science
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/190593
作者单位	Department of Chemical Engineering, Pennsylvania State University, University Park, PA 16802, United States; Center for Polymers and Organic Solids, University of California at Santa Barbara, Santa Barbara, CA 93106, United States
推荐引用方式 GB/T 7714	Saboe P.O.,Conte E.,Farell M.,et al. Biomimetic and bioinspired approaches for wiring enzymes to electrode interfaces[J],2017,10(1).
APA	Saboe P.O.,Conte E.,Farell M.,Bazan G.C.,&Kumar M..(2017).Biomimetic and bioinspired approaches for wiring enzymes to electrode interfaces.Energy & Environmental Science,10(1).
MLA	Saboe P.O.,et al."Biomimetic and bioinspired approaches for wiring enzymes to electrode interfaces".Energy & Environmental Science 10.1(2017).