气候变化领域集成服务门户(CCPortal): An experimental and theoretical study of an efficient polymer nano-photocatalyst for hydrogen evolution

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DOI	10.1039/c7ee00751e
	An experimental and theoretical study of an efficient polymer nano-photocatalyst for hydrogen evolution
	Pati P.B.; Damas G.; Tian L.; Fernandes D.L.A.; Zhang L.; Pehlivan I.B.; Edvinsson T.; Araujo C.M.; Tian H.
发表日期	2017
ISSN	17545692
起始页码	1372
结束页码	1376
卷号	10 期号:6
英文摘要	In this work, we report a highly efficient organic polymer nano-photocatalyst for light driven proton reduction. The system renders an initial rate of hydrogen evolution up to 50 ± 0.5 mmol g-1 h-1, which is the fastest rate among all other reported organic photocatalysts. We also experimentally and theoretically prove that the nitrogen centre of the benzothiadiazole unit plays a crucial role in the photocatalysis and that the Pdots structure holds a close to ideal geometry to enhance the photocatalysis. © The Royal Society of Chemistry 2017.
英文关键词	Catalysis; Organic polymers; Photocatalysis; Benzothiadiazoles; Hydrogen evolution; Ideal geometry; Initial rate; Light driven; Nano photocatalysts; Proton reduction; Theoretical study; Photocatalysts; catalysis; catalyst; experimental study; geometry; hydrogen; nitrogen; photochemistry; polymer; theoretical study
语种	英语
来源期刊	Energy & Environmental Science
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/190478
作者单位	Physical Chemistry Division, Department of Chemistry, Ångström Laboratory, Uppsala University, Box 523, Uppsala, 751 20, Sweden; Materials Theory Division, Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, 751 20, Sweden; Department of Engineering Sciences-Solid State Physics, Uppsala University, Box 534, Uppsala, 75121, Sweden
推荐引用方式 GB/T 7714	Pati P.B.,Damas G.,Tian L.,et al. An experimental and theoretical study of an efficient polymer nano-photocatalyst for hydrogen evolution[J],2017,10(6).
APA	Pati P.B..,Damas G..,Tian L..,Fernandes D.L.A..,Zhang L..,...&Tian H..(2017).An experimental and theoretical study of an efficient polymer nano-photocatalyst for hydrogen evolution.Energy & Environmental Science,10(6).
MLA	Pati P.B.,et al."An experimental and theoretical study of an efficient polymer nano-photocatalyst for hydrogen evolution".Energy & Environmental Science 10.6(2017).