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DOI | 10.1039/c8ee00151k |
Analyzing the efficiency, stability and cost potential for fullerene-free organic photovoltaics in one figure of merit | |
Li N.; McCulloch I.; Brabec C.J. | |
发表日期 | 2018 |
ISSN | 17545692 |
起始页码 | 1355 |
结束页码 | 1361 |
卷号 | 11期号:6 |
英文摘要 | The power conversion efficiencies (PCEs) of solution-processed organic photovoltaic (OPV) devices continue increasing towards the 15% milestone. Recently-emerging non-fullerene acceptors (NFAs) have significantly accelerated this development. Most of the efficiency analyses performed previously are based on a fullerene acceptor without considering its contribution to the enhancement of photo-absorption and PCE. Moreover, the stability and cost potential of OPV devices are usually not discussed, which sometimes makes the efficiency prediction less representative for broad interest. In this work, we effectively combine the prediction of efficiencies with experimentally determined stability data to analyze and predict the commercial potential of a NFA-based OPV product. Assuming that NFAs dominate the blend near IR absorption, the efficiency limit of OPV devices is predicted to be close to 20% and is found to be insensitive to the donor bandgap. With the excellent photo-stability observed for state-of-the-art NFA-based OPV devices, it is suggested that the corresponding customized donors with promising processing properties, excellent environmental stability and low synthesis complexity be designed as realistic material pairs for large-scale production and commercialization. © 2018 The Royal Society of Chemistry. |
英文关键词 | Forecasting; Fullerenes; Image enhancement; Nanostructured materials; Stability; Commercial potential; Efficiency predictions; Environmental stability; Large scale productions; Organic photovoltaic devices; Organic photovoltaics; Power conversion efficiencies; Processing properties; Efficiency; absorption; cost; efficiency measurement; energy efficiency; fullerene; photovoltaic system |
语种 | 英语 |
来源期刊 | Energy & Environmental Science
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/190235 |
作者单位 | Institute of Materials for Electronics and Energy Technology (I-MEET), Friedrich-Alexander University Erlangen-Nürnberg, Martensstraße 7, Erlangen, 91058, Germany; King Abdullah University of Science and Technology, KSC, Thuwal, 23955-6900, Saudi Arabia; Department of Chemistry and Centre for Plastic Electronics, Imperial College London, London, SW7 2AZ, United Kingdom; Bavarian Center for Applied Energy Research (ZAE Bayern), Immerwahrstraße 2, Erlangen, 91058, Germany |
推荐引用方式 GB/T 7714 | Li N.,McCulloch I.,Brabec C.J.. Analyzing the efficiency, stability and cost potential for fullerene-free organic photovoltaics in one figure of merit[J],2018,11(6). |
APA | Li N.,McCulloch I.,&Brabec C.J..(2018).Analyzing the efficiency, stability and cost potential for fullerene-free organic photovoltaics in one figure of merit.Energy & Environmental Science,11(6). |
MLA | Li N.,et al."Analyzing the efficiency, stability and cost potential for fullerene-free organic photovoltaics in one figure of merit".Energy & Environmental Science 11.6(2018). |
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