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| DOI | 10.1039/c8ee00162f |
| Introducing paired electric dipole layers for efficient and reproducible perovskite solar cells | |
| Lee J.-H.; Kim J.; Kim G.; Shin D.; Jeong S.Y.; Lee J.; Hong S.; Choi J.W.; Lee C.-L.; Kim H.; Yi Y.; Lee K. | |
| 发表日期 | 2018 |
| ISSN | 17545692 |
| 起始页码 | 1742 |
| 结束页码 | 1751 |
| 卷号 | 11期号:7 |
| 英文摘要 | Elimination of charge trapping at defects is highly challenging for poly-crystalline organometal halide perovskites. Here, we report a new architecture for reinforcing the built-in electric field (Ein) across the photoactive layer with a pair of strong electric dipole layers (EDLs). The paired EDLs significantly intensify the Ein across the perovskite layer, resulting in suppressed charge trapping of photogenerated charges. As a result, our low-temperature processed P-I-N planar PeSC devices using the paired EDLs exhibit a higher power conversion efficiency (ηmax ∼ 19.4%) and a smaller device-to-device variation with a standard deviation (S.D.) of 0.70%, which far surpass those (ηmax ∼ 17.8%, S.D. ∼ 1.1%) of the devices with typical charge transport layers. © 2018 The Royal Society of Chemistry. |
| 英文关键词 | Charge trapping; Electric fields; Heterojunction bipolar transistors; Perovskite; Solar cells; Temperature; Built-in electric fields; Charge transport layer; Electric dipole layer; Halide perovskites; Photoactive layers; Photogenerated charge; Power conversion efficiencies; Standard deviation; Perovskite solar cells; efficiency measurement; electric field; equipment; fuel cell; low temperature; perovskite; polymer; temperature effect |
| 语种 | 英语 |
| 来源期刊 | Energy & Environmental Science
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| 文献类型 | 期刊论文 |
| 条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/190202 |
| 作者单位 | School of Materials Science and Engineering, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea; Heeger Center for Advanced Materials, Research Institute for Solar and Sustainable Energies, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea; Institute of Physics and Applied Physics, Van der Waals Materials Research Center, Yonsei University, Seoul, 03722, South Korea; Advanced Photonics Research Institute, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea; Institute of Integrated Technology, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea; Department of Electrical and Computer Engineering, University of Toronto, 10 King's College Road, Toronto, ON M5S 3G4, Canada |
| 推荐引用方式 GB/T 7714 | Lee J.-H.,Kim J.,Kim G.,et al. Introducing paired electric dipole layers for efficient and reproducible perovskite solar cells[J],2018,11(7). |
| APA | Lee J.-H..,Kim J..,Kim G..,Shin D..,Jeong S.Y..,...&Lee K..(2018).Introducing paired electric dipole layers for efficient and reproducible perovskite solar cells.Energy & Environmental Science,11(7). |
| MLA | Lee J.-H.,et al."Introducing paired electric dipole layers for efficient and reproducible perovskite solar cells".Energy & Environmental Science 11.7(2018). |
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