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DOI10.1029/2021JC017239
Mechanisms Driving Decadal Changes in the Carbonate System of a Coastal Plain Estuary
Da F.; Friedrichs M.A.M.; St-Laurent P.; Shadwick E.H.; Najjar R.G.; Hinson K.E.
发表日期2021
ISSN21699275
卷号126期号:6
英文摘要Understanding decadal changes in the coastal carbonate system is essential for predicting how the health of these waters responds to anthropogenic drivers, such as changing atmospheric conditions and riverine inputs. However, studies that quantify the relative impacts of these drivers are lacking. In this study, the primary drivers of decadal trends in the surface carbonate system, and the spatiotemporal variability in these trends, are identified for a large coastal plain estuary: the Chesapeake Bay. Experiments using a coupled three-dimensional hydrodynamic-biogeochemical model highlight that, over the past three decades, the changes in the surface carbonate system of Chesapeake Bay have strong seasonal and spatial variability. The greatest surface pH and aragonite saturation state (ΩAR) reductions have occurred in the summer in the middle (mesohaline) Bay: −0.24 and −0.9 per 30 years, respectively, with increases in atmospheric CO2 and reductions in nitrate loading both being primary drivers. Reductions in nitrate loading have a strong seasonal influence on the carbonate system, with the most pronounced decadal decreases in pH and ΩAR occurring during the summer when primary production is strongly dependent on nutrient availability. Increases in riverine total alkalinity and dissolved inorganic carbon have raised surface pH in the upper oligohaline Bay, while other drivers such as atmospheric warming and input of acidified ocean water through the Bay mouth have had comparatively minor impacts on the estuarine carbonate system. This work has significant implications for estuarine ecosystem services, which are typically most sensitive to surface acidification in the spring and summer seasons. © 2021. The Authors.
英文关键词anthropogenic drivers; carbonate system; Chesapeake Bay; coastal acidification; decadal trends
语种英语
来源期刊Journal of Geophysical Research: Oceans
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/186277
作者单位Virginia Institute of Marine Science, William & Mary, Gloucester Point, VA, United States; CSIRO Oceans and Atmosphere, Hobart, TAS, Australia; Department of Meteorology and Atmospheric Science, The Pennsylvania State University, University ParkPA, United States
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Da F.,Friedrichs M.A.M.,St-Laurent P.,et al. Mechanisms Driving Decadal Changes in the Carbonate System of a Coastal Plain Estuary[J],2021,126(6).
APA Da F.,Friedrichs M.A.M.,St-Laurent P.,Shadwick E.H.,Najjar R.G.,&Hinson K.E..(2021).Mechanisms Driving Decadal Changes in the Carbonate System of a Coastal Plain Estuary.Journal of Geophysical Research: Oceans,126(6).
MLA Da F.,et al."Mechanisms Driving Decadal Changes in the Carbonate System of a Coastal Plain Estuary".Journal of Geophysical Research: Oceans 126.6(2021).
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