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DOI10.1029/2019JD032004
Fluxes of Atmospheric Greenhouse-Gases in Maryland (FLAGG-MD): Emissions of Carbon Dioxide in the Baltimore, MD-Washington, D.C. Area
Ahn D.Y.; Hansford J.R.; Howe S.T.; Ren X.R.; Salawitch R.J.; Zeng N.; Cohen M.D.; Stunder B.; Salmon O.E.; Shepson P.B.; Gurney K.R.; Oda T.; Lopez-Coto I.; Whetstone J.; Dickerson R.R.
发表日期2020
ISSN2169897X
卷号125期号:9
英文摘要To study emissions of CO2 in the Baltimore, MD-Washington, D.C. (Balt-Wash) area, an aircraft campaign was conducted in February 2015, as part of the Fluxes of Atmospheric Greenhouse-Gases in Maryland (FLAGG-MD) project. During the campaign, elevated mole fractions of CO2 were observed downwind of the urban center and local power plants. Upwind flight data and Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model analyses help account for the impact of emissions outside the Balt-Wash area. The accuracy, precision, and sensitivity of CO2 emissions estimates based on the mass balance approach were assessed for both power plants and cities. Our estimates of CO2 emissions from two local power plants agree well with their Continuous Emissions Monitoring Systems (CEMS) records. For the 16 power plant plumes captured by the aircraft, the mean percentage difference of CO2 emissions was -0.3%. For the Balt-Wash area as a whole, the 1σ CO2 emission rate uncertainty for any individual aircraft-based mass balance approach experiment was ±38%. Treating the mass balance experiments, which were repeated seven times within 9 days, as individual quantifications of the Balt-Wash CO2 emissions, the estimation uncertainty was ±16% (standard error of the mean at 95% CL). Our aircraft-based estimate was compared to various bottom-up fossil fuel CO2 (FFCO2) emission inventories. Based on the FLAGG-MD aircraft observations, we estimate 1.9 ± 0.3 MtC of FFCO2 from the Balt-Wash area during the month of February 2015. The mean estimate of FFCO2 from the four bottom-up models was 2.2 ± 0.3 MtC. ©2020. American Geophysical Union. All Rights Reserved.
英文关键词aircraft campaign; Baltimore-Washington, DC; carbon dioxide; CO2; greenhouse gas; urban emissions
语种英语
来源期刊Journal of Geophysical Research: Atmospheres
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/186013
作者单位Department of Chemistry and Biochemistry, University of Maryland, College Park, MD, United States; Department of Computer Science, University of Maryland, College Park, MD, United States; Department of Atmospheric and Oceanic Science, University of Maryland, College Park, MD, United States; Now at Areté, Arlington, VA, United States; Earth System Science Interdisciplinary Center, University of Maryland, College Park, MD, United States; National Oceanic and Atmospheric Administration Air Resource Laboratory, College Park, MD, United States; Department of Chemistry, Purdue University, West Lafayette, IN, United States; Now at Lake Michigan Air Directors Consortium, Madison, WI, United States; School of Marine and Atmospheric Sciences, Stony Brook University, Stony Brook, NY, United States; School of Informatics, Computing, and Cyber Systems, Northern Arizona University, Flagstaff, AZ, United States; Global Modeling and Assimilation Office, NASA Goddard Space Flight Center, Greenbelt, MD, United States; Godd...
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Ahn D.Y.,Hansford J.R.,Howe S.T.,et al. Fluxes of Atmospheric Greenhouse-Gases in Maryland (FLAGG-MD): Emissions of Carbon Dioxide in the Baltimore, MD-Washington, D.C. Area[J],2020,125(9).
APA Ahn D.Y..,Hansford J.R..,Howe S.T..,Ren X.R..,Salawitch R.J..,...&Dickerson R.R..(2020).Fluxes of Atmospheric Greenhouse-Gases in Maryland (FLAGG-MD): Emissions of Carbon Dioxide in the Baltimore, MD-Washington, D.C. Area.Journal of Geophysical Research: Atmospheres,125(9).
MLA Ahn D.Y.,et al."Fluxes of Atmospheric Greenhouse-Gases in Maryland (FLAGG-MD): Emissions of Carbon Dioxide in the Baltimore, MD-Washington, D.C. Area".Journal of Geophysical Research: Atmospheres 125.9(2020).
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