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DOI10.1029/2020JD032666
n-Alkanes and PAHs in the Southeastern Tibetan Plateau: Characteristics and Correlations With Brown Carbon Light Absorption
Zhu C.-S.; Li L.-J.; Huang H.; Dai W.-T.; Lei Y.-L.; Qu Y.; Huang R.-J.; Wang Q.-Y.; Shen Z.-X.; Cao J.-J.
发表日期2020
ISSN2169897X
卷号125期号:19
英文摘要The samples of atmospheric total suspended particle (TSP) were obtained at the remote Tibetan site (named Lulang) from November 2015 to November 2016. The seasonal characteristics of n-alkanes, polycyclic aromatic hydrocarbons (PAHs) variations, and their correlations to brown carbon (BrC) light absorption in TSP were investigated. Elevated TSP n-alkanes and PAHs levels were observed in winter (2.8 and 10 times higher than in monsoon, respectively), largely due to the seasonal contributions of wintertime home heating and long-range transport. The total-PAHs was found to correlate strongly with the methanol-soluble BrC (MeS-BrC) light absorption coefficient (babs) (R = 0.80) compared to water-soluble BrC (WS-BrC) (R = 0.70) at 365 nm. The BrC solar absorptions percentages to those of element carbon (EC) in the range of ultraviolet (300–400 nm) were high in both winter and premonsoon seasons, which can affect the vulnerable environmental radiative balance and atmospheric photochemistry. ©2020. American Geophysical Union. All Rights Reserved.
英文关键词brown carbon; correlation analysis; n-alkanes; PAHs; the Tibetan Plateau
语种英语
来源期刊Journal of Geophysical Research: Atmospheres
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/185711
作者单位Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, China; CAS Center for Excellence in Quaternary Science and Global Change, Xi'an, China; School of Resource, Environmental and Chemical Engineering, Nanchang University, Nanchang, China; Department of Environmental Science and Engineering, Xi'an Jiaotong University, Xi'an, China
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Zhu C.-S.,Li L.-J.,Huang H.,et al. n-Alkanes and PAHs in the Southeastern Tibetan Plateau: Characteristics and Correlations With Brown Carbon Light Absorption[J],2020,125(19).
APA Zhu C.-S..,Li L.-J..,Huang H..,Dai W.-T..,Lei Y.-L..,...&Cao J.-J..(2020).n-Alkanes and PAHs in the Southeastern Tibetan Plateau: Characteristics and Correlations With Brown Carbon Light Absorption.Journal of Geophysical Research: Atmospheres,125(19).
MLA Zhu C.-S.,et al."n-Alkanes and PAHs in the Southeastern Tibetan Plateau: Characteristics and Correlations With Brown Carbon Light Absorption".Journal of Geophysical Research: Atmospheres 125.19(2020).
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