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DOI | 10.1038/s41612-018-0056-2 |
Evidence of major secondary organic aerosol contribution to lensing effect black carbon absorption enhancement | |
Zhang Y.; Favez O.; Canonaco F.; Liu D.; Močnik G.; Amodeo T.; Sciare J.; Prévôt A.S.H.; Gros V.; Albinet A. | |
发表日期 | 2018 |
ISSN | 23973722 |
卷号 | 1期号:1 |
英文摘要 | Atmospheric black carbon (BC) has a strong positive, but still controversial, effect on global warming. In particular, BC absorption enhancement (Eabs) due to internal mixing with other chemical species—so-called lensing effect—is poorly assessed. This bottleneck partly relies on the lack of long-term in situ measurements of both the optical and chemical properties of BC-containing particles. Here, we present experimental and computational results showing a significant Eabs increase with the aerosol photochemical aging. This was associated with the production of highly oxidized secondary organic aerosols (SOA), especially at summertime. The 3-year-long continuous aerosol chemical and optical measurements used for the present study was obtained in the Paris region, France, which might be representative of near-future air quality within developing countries. These findings suggest that SOA could represent one of the most critical chemical species to be considered within climate models. © 2018, The Author(s). |
语种 | 英语 |
scopus关键词 | absorption; aerosol; air quality; black carbon; concentration (composition); global warming; seasonal variation; France; Ile de France; Paris; Ville de Paris |
来源期刊 | npj Climate and Atmospheric Science
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/178169 |
作者单位 | Institut National de l’Environnement Industriel et des Risques, Verneuil-en-Halatte, France; Laboratoire des Sciences du Climat et de l’Environnement, CNRS-CEA-UVSQ, Gif-sur-Yvette, France; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland; Centre for Atmospheric Sciences, School of Earth and Environmental Sciences, University of Manchester, Manchester, United Kingdom; Condensed Matter Physics Department, J. Stefan Institute, Ljubljana, Slovenia; Environment Energy and Water Research Center, The Cyprus Institute, Nicosia, Cyprus |
推荐引用方式 GB/T 7714 | Zhang Y.,Favez O.,Canonaco F.,et al. Evidence of major secondary organic aerosol contribution to lensing effect black carbon absorption enhancement[J],2018,1(1). |
APA | Zhang Y..,Favez O..,Canonaco F..,Liu D..,Močnik G..,...&Albinet A..(2018).Evidence of major secondary organic aerosol contribution to lensing effect black carbon absorption enhancement.npj Climate and Atmospheric Science,1(1). |
MLA | Zhang Y.,et al."Evidence of major secondary organic aerosol contribution to lensing effect black carbon absorption enhancement".npj Climate and Atmospheric Science 1.1(2018). |
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