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DOI10.1016/j.fuel.2019.115627
Utilization of CO2 in renewable DME fuel production: A life cycle analysis (LCA)-based case study in China
Tomatis M.; Mahmud Parvez A.; Afzal M.T.; Mareta S.; Wu T.; He J.; He T.
发表日期2019
ISSN162361
卷号254
英文摘要This work aimed to evaluate the environmental performance of single-step dimethyl ether (DME) production system through CO2-enhanced gasification of gumwood. The proposed CO2-enhanced gasification based bio-DME production process was compared systematically with the conventional approach in terms of life cycle assessment (LCA) impacts by using SimaPro software. Overall, the LCA results revealed that bio-DME fuel produced from CO2-enhanced process significantly reduced the burden on climate change, toxicity and eco-toxicity by at least 20%. This decrement was mostly attributed to low feedstock consumption, high-energy recovery and CO2 utilization in the CO2-enhanced process. Over 53% contribution in all impact categories were contributed by the gasifier unit, mainly due to its high energy intensity (over 60% of the total energy requirement). Moreover, the effect of replacing diesel by bio-DME or diesel/DME blend as an automotive fuel was assessed in this study. The scenario of using pure DME resulted on significant reductions of greenhouse gas (GHG) emissions, by 72%, and of its impact on both human health and ecosystem (by 55% and 68%, respectively). The reduction of GHG emissions were caused by the carbon neutrality of bio-DME. Utilization of DME also limited the emissions of carcinogenic particulate such as diesel soot and therefore, decreased the toxicity of traffic emissions. The second scenario was to utilize DME15 (15% DME by wt in diesel) as an automotive fuel. However, only minor decreases, up to 7%, of the environmental impact were observed for DME15 compared to those estimated for pure diesel. Thus, the present study demonstrated that the CO2-enhanced process could greatly reduce GHG emission and environmental burden of DME production compared to the conventional method. Furthermore, bio-DME utilization as fuel for automotive applications can significantly decrease the hazard caused by traffic emissions. Elsevier Ltd
英文关键词Bio-DME; CO2-enhanced gasification; Diesel; DME15; Fuel replacement; LCA
scopus关键词Artificial life; Automotive fuels; Biohazards; Carbon dioxide; Climate change; Diesel engines; Environmental impact; Environmental management; Gas emissions; Gasification; Greenhouse gases; Toxicity; Automotive applications; Bio DME; Conventional approach; Diesel; DME15; Environmental performance; Life Cycle Assessment (LCA); Total energy requirement; Life cycle
来源期刊Fuel
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/176166
作者单位Department of Chemical and Environmental Engineering, The University of Nottingham Ningbo China, Ningbo, 315100, China; Department of Mechanical Engineering, University of New Brunswick, 15 Dineen Drive, Fredericton, E3B 5A3, Canada; Centre for English Language Education (CELE), The University of Nottingham Ningbo China, Ningbo, 315100, China; Department of Gas Engineering, College of Pipeline and Civil Engineering, China University of Petroleum (East China), Qingdao, 266580, China
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Tomatis M.,Mahmud Parvez A.,Afzal M.T.,et al. Utilization of CO2 in renewable DME fuel production: A life cycle analysis (LCA)-based case study in China[J],2019,254.
APA Tomatis M..,Mahmud Parvez A..,Afzal M.T..,Mareta S..,Wu T..,...&He T..(2019).Utilization of CO2 in renewable DME fuel production: A life cycle analysis (LCA)-based case study in China.Fuel,254.
MLA Tomatis M.,et al."Utilization of CO2 in renewable DME fuel production: A life cycle analysis (LCA)-based case study in China".Fuel 254(2019).
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