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DOI10.1039/c9ee03930a
Transforming energy using quantum dots
Lu H.; Huang Z.; Martinez M.S.; Johnson J.C.; Luther J.M.; Beard M.C.
发表日期2020
ISSN1754-5692
起始页码1347
结束页码1376
卷号13期号:5
英文摘要Colloidal quantum dots (QDs) have emerged as versatile and efficient scaffolds to absorb light and then manipulate, direct, and convert that energy into other useful forms of energy. The QD characteristics (optical, electrical, physical) can be readily tuned via solution phase chemistries in order to affect the flow of energy, initially contained in the photons of light, using rational design. Key parameters under control are the size and shape, internal composition (e.g., alloys, core/shell heterostructures, semiconductor/metal interfaces), surface composition (ligand chemistries), and film composition (e.g., QD-QD electronic coupling, bulk heterostructure formation, QD/biological interfaces). In this review, we summarize recent progress using QDs in energy conversion architectures with the express goal of transforming optical energy to other forms of energy, including electricity, photons with different energies, and chemical bonds, i.e., photovoltaics, photon up- or down-conversion, and photocatalytic process, respectively. The advantages of using QDs in absorbing and then directing and converting optical energy over molecular chromophores are highlighted. Finally, we discuss ongoing challenges and opportunities associated with using QDs for absorbing, manipulating and directing the flow of energy. © The Royal Society 2020 of Chemistry.
语种英语
scopus关键词Bond strength (chemical); Chromophores; Energy conversion; Heterojunctions; Light; Nanocrystals; Photons; Quantum chemistry; Scaffolds; Sols; Colloidal quantum dots; Electronic coupling; Film composition; Internal composition; Ligand chemistry; Photocatalytic process; Recent progress; Solution-phase chemistry; Semiconductor quantum dots; energy budget; energy conservation; quantitative analysis
来源期刊Energy and Environmental Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/162656
作者单位Chemistry and Nanoscience Center, National Renewable Energy Laboratory, Golden, CO 80401, United States
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GB/T 7714
Lu H.,Huang Z.,Martinez M.S.,et al. Transforming energy using quantum dots[J],2020,13(5).
APA Lu H.,Huang Z.,Martinez M.S.,Johnson J.C.,Luther J.M.,&Beard M.C..(2020).Transforming energy using quantum dots.Energy and Environmental Science,13(5).
MLA Lu H.,et al."Transforming energy using quantum dots".Energy and Environmental Science 13.5(2020).
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