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DOI10.1029/98JD01802
Soluble species in aerosol and snow and their relationship at Glacier 1, Tien Shan, China
Sun, JY; Qin, DH; Mayewski, PA; Dibb, JE; Whitlow, S; Li, ZQ; Yang, QZ
发表日期1998
ISSN2169-897X
起始页码28021
结束页码28028
卷号103期号:D21
英文摘要Simultaneous sampling of aerosol (n = 20) and snow (n = 114) was made at Glacier 1, Tien Shan, between May 19 and June 29, 1996. Similar temporal patterns of some major ion (calcium, magnesium, potassium, Sodium, chloride, and sulfate) concentrations between snow and aerosol show that snow chemistry basically reflects changes in the chemistry of the atmosphere. This gives us confidence in the reconstruction of past atmospheric change using some snow data. There are no significant correlations between aerosol and snow samples for ammonium and nitrate. This suggests that postdepositional and/or postcollection processes may alter ammonium and nitrate concentrations in snow. The fact that the measured cations in aerosol and snow always exceed the measured anions suggests that the atmosphere is alkaline over Glacier 1? Tien Shan. In aerosol and snow samples, calcium is the dominant cationic species, with sulfate and presumed carbonate being the dominant anions. There ii a very good inverse relationship (r = 0.96) between the equivalence ratio of calcium to sulfate and the ratio of ammonium to sulfate in aerosols, but this relationship does not hold for snow. This further suggests that postdepositional and/or postcollection processes exert important controls on ammonium concentrations in snow. Although melt-freeze cycles might increase the concentration of all crustal species through progressive dissolution of dust, these cycles seem most important for magnesium and carbonate.
WOS研究方向Meteorology & Atmospheric Sciences
WOS类目Meteorology & Atmospheric Sciences
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/158776
作者单位Sun, JY (corresponding author), Chinese Acad Sci, Lanzhou Inst Glaciol & Geocryol, Lab Ice Core & Cold Reg Environm, Lanzhou 730000, Peoples R China.
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Sun, JY,Qin, DH,Mayewski, PA,et al. Soluble species in aerosol and snow and their relationship at Glacier 1, Tien Shan, China[J],1998,103(D21).
APA Sun, JY.,Qin, DH.,Mayewski, PA.,Dibb, JE.,Whitlow, S.,...&Yang, QZ.(1998).Soluble species in aerosol and snow and their relationship at Glacier 1, Tien Shan, China.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,103(D21).
MLA Sun, JY,et al."Soluble species in aerosol and snow and their relationship at Glacier 1, Tien Shan, China".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 103.D21(1998).
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