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DOI | 10.5194/acp-20-7929-2020 |
Source apportionment of atmospheric mercury in the remote marine atmosphere: Mace Head GAW station, Irish western coast | |
Custodio D.; Ebinghaus R.; Gerard Spain T.; Bieser J. | |
发表日期 | 2020 |
ISSN | 16807316 |
起始页码 | 7929 |
结束页码 | 7939 |
卷号 | 20期号:13 |
英文摘要 | We examined recent atmospheric mercury concentrations measured with a high temporal resolution of 15 min at Mace Head, a GAW station on the western coast of Ireland. We attributed a direct contribution of 34 % (0.44 ng m-3) to primary sources. Additionally, a steep decline (0.05 ng yr-1) in mercury concentrations was observed between 2013 and 2018. Using a stereo algorithm we reconstructed 99.9 % of the atmospheric mercury. A conservative analysis demonstrated no decrease in total gaseous mercury (TGM) associated with atmospheric species typically used as tracers for oceanic emissions. The results show that the atmospheric mercury mass is mainly loaded in a baseline factor with an ongoing decline. Moreover, we exploit temporal variation and wind pattern effects in the measured atmospheric species; the results show that the diurnal variation and seasonality in TGM observed in Mace Head are closely related to other species linked to primary sources and can be explained by transport from continental areas. © Author(s) 2020. This work is distributed under the Creative Commons Attribution 4.0 License. |
语种 | 英语 |
scopus关键词 | algorithm; atmospheric pollution; concentration (composition); marine atmosphere; mercury (element); pollutant transport; source apportionment; temporal variation; wind forcing; Connacht; Galway [(CNT) Connacht]; Ireland; Mace Head |
来源期刊 | Atmospheric Chemistry and Physics |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/152880 |
作者单位 | Helmholtz-Zentrum Geesthacht, Institute of Coastal Research, Max-Planck-Str. 1, Geesthacht, 21502, Germany; National University of Ireland, Galway, Ireland |
推荐引用方式 GB/T 7714 | Custodio D.,Ebinghaus R.,Gerard Spain T.,et al. Source apportionment of atmospheric mercury in the remote marine atmosphere: Mace Head GAW station, Irish western coast[J],2020,20(13). |
APA | Custodio D.,Ebinghaus R.,Gerard Spain T.,&Bieser J..(2020).Source apportionment of atmospheric mercury in the remote marine atmosphere: Mace Head GAW station, Irish western coast.Atmospheric Chemistry and Physics,20(13). |
MLA | Custodio D.,et al."Source apportionment of atmospheric mercury in the remote marine atmosphere: Mace Head GAW station, Irish western coast".Atmospheric Chemistry and Physics 20.13(2020). |
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