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DOI | 10.1016/j.atmosenv.2020.117741 |
VOC characteristics and sources at nine photochemical assessment monitoring stations in western Taiwan | |
Huang Y.S.; Hsieh C.C. | |
发表日期 | 2020 |
ISSN | 13522310 |
卷号 | 240 |
英文摘要 | Using 2017 data, 54 volatile organic compounds (VOCs) in Taiwan's atmospheric environment from nine photochemical assessment monitoring stations (PAMSs) were collected and their characteristics and sources were analyzed. High VOC concentration spots were exposed in urban and industrial areas (Wanhua, Tucheng, Chungming, Tainan, Qiaotou, and Xiaogang). The major categories of VOC were alkanes and aromatics. Among them, benzene, toluene, ethylbenzene, and m,p-xylene (BTEX) predominated and contributed to ozone formation potential (OFP) and secondary organic aerosol formation (SOAF). T/B and X/E ratios showed that VOCs in urban and industrial areas originated from fresh, mixed sources of local emissions. Positive matrix factorization (PMF) analysis indicated that industrial emissions (solvent usage, industry, and petrochemical plant) were the primary contributors, followed secondarily by traffic emissions (vehicular emission and vehicular fuel evaporation), and aged air-mass. Analysis by potential source contribution function (PSCF) was conducted to confirm the effects of aged air-mass sources. The estimated VOC sources OFP and SOAF indicated that industrial emissions were the greatest contributors to OFP and SOAF. Results from this study imply that VOC control measures should prioritize control of industrial emissions. © 2020 |
英文关键词 | BTEX ratio; Ozone formation potential; Positive matrix factorization; Potential source contribution function; Secondary organic aerosol potential |
语种 | 英语 |
scopus关键词 | Factorization; Petrochemical plants; Volatile organic compounds; Atmospheric environment; Ozone formation potentials; Photochemical assessment monitoring stations; Positive Matrix Factorization; Potential source contribution function; Secondary organic aerosols; Traffic emissions; Vehicular emission; Industrial emissions; alkane; alkane derivative; aromatic compound; benzene; ethylbenzene; toluene; volatile organic compound; xylene; aerosol formation; assessment method; chemical compound; monitoring; photochemistry; pollutant source; pollution control; volatile organic compound; air quality; Article; environmental protection; industrial area; photochemistry; priority journal; quality control; secondary organic aerosol; Taiwan; urban area; Tainan; Taiwan |
来源期刊 | Atmospheric Environment
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/144977 |
作者单位 | Department and Graduate School of Safety Health and Environment Engineering, National Yunlin University of Science and Technology, Yunlin, 64002, Taiwan |
推荐引用方式 GB/T 7714 | Huang Y.S.,Hsieh C.C.. VOC characteristics and sources at nine photochemical assessment monitoring stations in western Taiwan[J],2020,240. |
APA | Huang Y.S.,&Hsieh C.C..(2020).VOC characteristics and sources at nine photochemical assessment monitoring stations in western Taiwan.Atmospheric Environment,240. |
MLA | Huang Y.S.,et al."VOC characteristics and sources at nine photochemical assessment monitoring stations in western Taiwan".Atmospheric Environment 240(2020). |
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