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DOI10.5194/acp-19-1819-2019
The influence of transformed Reynolds number suppression on gas transfer parameterizations and global DMS and CO2 fluxes
Zavarsky A.; Marandino C.A.
发表日期2019
ISSN16807316
起始页码1819
结束页码1834
卷号19期号:3
英文摘要Eddy covariance measurements show gas transfer velocity suppression at medium to high wind speed. A wind- wave interaction described by the transformed Reynolds number is used to characterize environmental conditions favoring this suppression. We take the transformed Reynolds number parameterization to review the two most cited wind speed gas transfer velocity parameterizations: Nightingale et al. (2000) and Wanninkhof (1992, 2014). We propose an algorithm to adjust k values for the effect of gas transfer suppression and validate it with two directly measured dimethyl sulfide (DMS) gas transfer velocity data sets that experienced gas transfer suppression. We also show that the data set used in the Nightingale 2000 parameterization experienced gas transfer suppression. A compensation of the suppression effect leads to an average increase of 22% in the k vs. u relationship. Performing the same correction forWanninkhof 2014 leads to an increase of 9.85 %. Additionally, we applied our gas transfer suppression algorithm to global air- sea flux climatologies of CO2 and DMS. The global application of gas transfer suppression leads to a decrease of 11% in DMS outgassing. We expect the magnitude of Reynolds suppression on any global air-sea gas exchange to be about 10 %. © 2019 Author(s).
语种英语
scopus关键词atmosphere-ocean coupling; carbon dioxide; data set; dimethylsulfide; flux measurement; gas exchange; parameterization; Reynolds number
来源期刊Atmospheric Chemistry and Physics
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/144651
作者单位Independent Researcher, Kiel, Germany; GEOMAR Helmholtz Centre for Ocean Research, Kiel, Germany
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Zavarsky A.,Marandino C.A.. The influence of transformed Reynolds number suppression on gas transfer parameterizations and global DMS and CO2 fluxes[J],2019,19(3).
APA Zavarsky A.,&Marandino C.A..(2019).The influence of transformed Reynolds number suppression on gas transfer parameterizations and global DMS and CO2 fluxes.Atmospheric Chemistry and Physics,19(3).
MLA Zavarsky A.,et al."The influence of transformed Reynolds number suppression on gas transfer parameterizations and global DMS and CO2 fluxes".Atmospheric Chemistry and Physics 19.3(2019).
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