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DOI | 10.1016/j.atmosres.2019.104762 |
On the chemical nature of wet deposition over a major desiccated lake: Case study for Lake Urmia basin | |
Ahmady-Birgani H.; Ravan P.; Schlosser J.S.; Cuevas-Robles A.; AzadiAghdam M.; Sorooshian A. | |
发表日期 | 2020 |
ISSN | 0169-8095 |
卷号 | 234 |
英文摘要 | One of the largest hyper-saline lakes in the world is Lake Urmia, which is in the northwest region of Iran. Lake Urmia has experienced extreme desiccation in recent years. This study was conducted to investigate possible impacts of aerosol emitted by Lake Urmia on rainwater properties. Rainwater samples were collected from September 2017 to September 2018 at 13 sites spanning different areas of the Lake Urmia basin. Samples were analysed for acidity/alkalinity (pH), electrical conductivity (EC), total suspended solids (TSS) and elemental composition (Na, Mg, K, Ca, Al, Fe, Ti, V, Cr, Mn, Co, Ni, Cu, Zn, As, Se, and Pb). The results reveal that rainwater around Lake Urmia is characterized by high concentrations of heavy metals and toxic elements (e.g., Fe, Al, Ni, Cu, Cr, Co, Ti), especially in the outer ring of the study region to the north. Chemical signatures of anthropogenic pollution were most evident at sites near populated and manufacturing centers. The average pH of rainwater was enhanced relative to other regions, with the lowest and highest values of the 13 sites being 7.7 and 8.6, respectively. Concentrations of marine elements (Na+, K+, Mg2+, Ca2+) decreased with increasing distance from Lake Urmia, suggestive of possible impacts of the lakebed's emission on rain composition via likely below-cloud scavenging. The area impacted by the marine aerosol emitted by Lake Urmia has a diameter of 30 to 40 km surrounding the shoreline. The results reveal a stronger signature of crustal species in the north owing to desiccated lakebed hotspots located in the north. © 2019 Elsevier B.V. |
英文关键词 | Aerosol; Atmospheric particulates; Chemical composition; Lake Urmia; Rainwater samples; Wet depositions |
学科领域 | Aerosols; Deposition; Heavy metals; Atmospheric particulate; Chemical compositions; Lake urmia; Rainwater samples; Wet deposition; Lakes; aerosol; chemical composition; desiccation; particulate matter; rainwater; wet deposition; Iran; Lake Urmia |
语种 | 英语 |
scopus关键词 | Aerosols; Deposition; Heavy metals; Atmospheric particulate; Chemical compositions; Lake urmia; Rainwater samples; Wet deposition; Lakes; aerosol; chemical composition; desiccation; particulate matter; rainwater; wet deposition; Iran; Lake Urmia |
来源期刊 | Atmospheric Research
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/120521 |
作者单位 | Faculty of Natural Resources, Urmia University, Urmia, Iran; Department of Chemical and Environmental Engineering, University of Arizona, Tucson, AZ, United States; Department of Hydrology and Atmospheric Sciences, University of Arizona, Tucson, AZ, United States |
推荐引用方式 GB/T 7714 | Ahmady-Birgani H.,Ravan P.,Schlosser J.S.,et al. On the chemical nature of wet deposition over a major desiccated lake: Case study for Lake Urmia basin[J],2020,234. |
APA | Ahmady-Birgani H.,Ravan P.,Schlosser J.S.,Cuevas-Robles A.,AzadiAghdam M.,&Sorooshian A..(2020).On the chemical nature of wet deposition over a major desiccated lake: Case study for Lake Urmia basin.Atmospheric Research,234. |
MLA | Ahmady-Birgani H.,et al."On the chemical nature of wet deposition over a major desiccated lake: Case study for Lake Urmia basin".Atmospheric Research 234(2020). |
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