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DOI10.1002/ese3.334
Effect of internal hydrocarbon reforming during coupled operation of a biomass gasifier with hot gas cleaning and SOFC stacks
Fischer, Felix1; Hauser, Michael1; Hauck, Maximilian1; Herrmann, Stephan1; Fendt, Sebastian1; Jeong, Hyeondeok2; Lenser, Christian2; Menzler, Norbert H.2; Spliethoff, Hartmut1,3
发表日期2019
ISSN2050-0505
卷号7期号:4页码:1140-1153
英文摘要

In the context of energy transition and climate change, a combination of highly efficient modern solid oxide fuel cells (SOFC) and thermo-chemical conversion of biogenic residues could complement other intermittent renewable sources such as wind and solar. In order to reduce required gas cleaning efforts and to increase the process efficiency, the influence of hydrocarbons on SOFC performance is experimentally investigated in this study. For the first time, the operation of Ni/YSZ anode-supported cells in Julich F10 stacks is performed with pre-reformed and with bio-syngas containing full hydrocarbon content at realistic current densities. Sulfur and other impurities were removed in both cases. No degradation could be observed within normal operation on clean gas. With the tar reformer bypassed, the pressure drop over the stack increased due to severe carbon deposition on the anode substrate and the nickel current collector mesh inside the SOFC stack, so that operation had to be terminated after five hours. This behavior is different from single-cell tests, where electrochemical degradation is the limiting factor. The results show that improvements are not only necessary for cell materials and that future research must also consider other stack components.


WOS研究方向Energy & Fuels
来源期刊ENERGY SCIENCE & ENGINEERING
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/101295
作者单位1.Tech Univ Munich, Chair Energy Syst, Garching, Germany;
2.Forschungszentrum Julich, Julich, Germany;
3.Bayer Zentrum Angew Energieforsch eV, Garching, Germany
推荐引用方式
GB/T 7714
Fischer, Felix,Hauser, Michael,Hauck, Maximilian,et al. Effect of internal hydrocarbon reforming during coupled operation of a biomass gasifier with hot gas cleaning and SOFC stacks[J],2019,7(4):1140-1153.
APA Fischer, Felix.,Hauser, Michael.,Hauck, Maximilian.,Herrmann, Stephan.,Fendt, Sebastian.,...&Spliethoff, Hartmut.(2019).Effect of internal hydrocarbon reforming during coupled operation of a biomass gasifier with hot gas cleaning and SOFC stacks.ENERGY SCIENCE & ENGINEERING,7(4),1140-1153.
MLA Fischer, Felix,et al."Effect of internal hydrocarbon reforming during coupled operation of a biomass gasifier with hot gas cleaning and SOFC stacks".ENERGY SCIENCE & ENGINEERING 7.4(2019):1140-1153.
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